材料科学
光致发光
量子点
发光
钙钛矿(结构)
光电子学
接触角
猝灭(荧光)
纳米技术
蒸发
激光器
光学
复合材料
化学工程
荧光
物理
工程类
热力学
作者
Ziyi Chen,Jun Chen,Teng Ma,Weishu Guo,Xiaojing Li,Jiancheng Lai,Haibo Zeng,Zhenhua Li
出处
期刊:Nano Letters
[American Chemical Society]
日期:2025-01-31
标识
DOI:10.1021/acs.nanolett.4c06610
摘要
Perovskite quantum dots (PQDs) have garnered significant attention in the display industry as high-performance luminescent materials in recent years. However, in outdoor applications, it is highly challenging to maintain the luminescent performance of PQDs while simultaneously ensuring superhydrophobicity and self-cleaning functionality in rainy weather conditions. Here, we report a luminescent pixel array fabricated using superhydrophobic PQDs with a photoluminescence quantum yield (PLQY) of 32%. The surface exhibits a high static contact angle of 168° and a rolling angle of <1°, demonstrating excellent self-cleaning ability. Specifically, by loading encapsulated PQDs onto fluorinated silica particles of varying particle sizes, a multilevel micronano hierarchical raspberry-like interface is formed. Simultaneously, local evaporation quenching induced by pulsed laser irradiation is employed to create a photoluminescent array with individual pixel diameters of 300 μm and a spacing of 80 μm. This achievement fills the gap in the application of PQDs for outdoor displays.
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