材料科学
碳纳米管
氮气
退火(玻璃)
兴奋剂
惰性气体
热稳定性
化学工程
惰性
纳米技术
检出限
分析化学(期刊)
复合材料
光电子学
化学
色谱法
有机化学
工程类
作者
Xiao-Han Tian,Tianya Zhou,Yu Meng,Yiming Zhao,Chao Shi,Peng‐Xiang Hou,Lili Zhang,Chang Liu,Hui‐Ming Cheng
出处
期刊:Molecules
[MDPI AG]
日期:2022-10-02
卷期号:27 (19): 6523-6523
被引量:6
标识
DOI:10.3390/molecules27196523
摘要
Carbon nanotubes (CNTs) are considered a promising candidate for the detection of toxic gases because of their high specific surface area and excellent electrical and mechanical properties. However, the detecting performance of CNT-based detectors needs to be improved because covalently bonded CNTs are usually chemically inert. We prepared a nitrogen-doped single-wall CNT (SWCNT) film by means of gas-phase fluorination followed by thermal annealing in NH3. The doped nitrogen content could be changed in the range of 2.9-9.9 at%. The N-doped SWCNT films were directly used to construct flexible and transparent gas sensors, which can work at a low voltage of 0.01 V. It was found that their NO2 detection performance was closely related to their nitrogen content. With an optimum nitrogen content of 9.8 at%, a flexible sensor had a detection limit of 500 ppb at room temperature with good cycling ability and stability during bending.
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