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Physicochemical Properties and Phosphorus Adsorption Capacity of Ceramsite Made from Alum Sludge

明矾 吸附 化学 比表面积 动力学 化学工程 浸出(土壤学) 朗缪尔吸附模型 材料科学 制浆造纸工业 催化作用 有机化学 环境科学 物理 量子力学 土壤科学 工程类 土壤水分
作者
Shi Li,Xiaohong Zhao,Yongxiang Cao,Hongjuan Ma,Xuejun Sun
出处
期刊:Water [Multidisciplinary Digital Publishing Institute]
卷期号:15 (13): 2427-2427 被引量:3
标识
DOI:10.3390/w15132427
摘要

Alum sludge is an inevitable by-product from the water purification process, which had been applied as substrates in some constructed wetlands with good performance, especially for phosphorus (P) adsorption. The raw alum sludge is similar to a clay lump with an irregular shape, and there is a concern of it leaching into water. For better reuse, herein, some sludge was fired to produce alum sludge ceramsite (ASC) with a uniform spherical shape via a four-step process of kneading the sludge ball, air drying, preheating at 400 °C for 10 min, and firing at 600 °C for 5 min. Meanwhile, an air-dried alum sludge ball (adASB) was manufactured for comparison. The physicochemical properties and P adsorption ability of ceramsite were investigated subsequently. Through XRD and FT-IR tests, there was no obvious difference between ASC and adASB on the phase structure, but there was a certain amount of Al-OH group loss on the surface of ASC. The structure of ASC was still amorphous, similar to adASB, while ASC possessed more micropore structure and a bigger specific surface area than adASB. Adsorption experiments showed the P adsorption behaviors of ASC and adASB were much similar, and their adsorption kinetics were in accordance with the two-step adsorption kinetics rate equation and pseudo-second-order kinetics equation. The maximum adsorption capacities of ASC and adASB fitted by the Langmuir model were 1.66 mg/g and 1.89 mg/g, respectively. It should be pointed out that, compared with other adsorbents, the ASC produced in this study still had a greater ability to adsorb P. Therefore, ASC should have a great application potential for P removal in wastewater treatment in China.
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