Organizing Photosensitive and Photothermal Single‐Sites Uniformly in a Trimetallic Metal‐Organic Framework for Efficient Photocatalytic Hydrogen Evolution

Effective combination of the photosensitivity and photothermal property in photocatalyst is vital to achieve the maximum light utilization for superior photocatalytic efficiency. Herein, this work successfully organizes photosensitive Cd-NS single-sites and photothermal Ni-NS single-sites uniformly at a molecular level within a tailored trimetallic metal-organic framework. The optimized Ho