3-D hierarchical micro/nano-structures of porous Bi2WO6: Controlled hydrothermal synthesis and enhanced photocatalytic performances

光催化 热液循环 材料科学 氧化剂 化学工程 水热合成 X射线光电子能谱 纳米技术 催化作用 多孔性 可见光谱 反应速率常数 化学 动力学 复合材料 有机化学 光电子学 物理 工程类 量子力学
作者
Zesheng Li,Meihua Luo,Bolin Li,Qiachun Lin,Xichun Liao,Huiqing Yu,Changlin Yu
出处
期刊:Microporous and Mesoporous Materials [Elsevier BV]
卷期号:313: 110830-110830 被引量:24
标识
DOI:10.1016/j.micromeso.2020.110830
摘要

As one of the simplest aurivillius layered materials, Bi2WO6 is a promising photocatalyst with a wide range of applications. The construction of 3-D hierarchical micro/nano-structures (3-D HMNSs) can be considered as an excellent strategy to improve the photocatalytic activity. In this paper, a series of porous Bi2WO6 photocatalysts with 3-D HMNSs were synthesized by hydrothermal method via adjusting the concentration of reactants. All kinds of characterization methods (XRD, SEM, TEM, BET, UV–Vis, etc.) were used to characterize the as-synthesized samples. Taking tetracycline as a model pollutant, the photocatalytic properties of these Bi2WO6 photocatalysts were investigated, and the mechanism of its photocatalytic degradation was also proposed. The Bi2WO6-4# sample showed the highest visible-light photocatalytic activity, with tetracycline removal rate of 99.9% in 1 h irradiation and a kinetic reaction rate constant of 0.06071 min−1. The catalytic mechanism analysis shows that the active radicals of ·OH and ·O2− produced by the photoelectron hole have strong oxidizing property, which can quickly decompose tetracycline. Bi2WO6-4# with oriented arrangement of nanocrystals and increased Eg have the advantage of promoting the separation of electron-hole pair, accounting for the high photocatalytic activity.
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