Recent progress on silicon-based anode materials for practical lithium-ion battery applications

材料科学 阳极 锂(药物) 工程物理 电池(电) 石墨 电解质 商业化 纳米技术 工艺工程 光电子学 复合材料 电极 工程类 物理化学 功率(物理) 化学 法学 内分泌学 物理 医学 量子力学 政治学
作者
Peng Li,Guoqiang Zhao,Xiaobo Zheng,Xun Xu,Chenghao Yao,Wenping Sun,Shi Xue Dou
出处
期刊:Energy Storage Materials [Elsevier]
卷期号:15: 422-446 被引量:358
标识
DOI:10.1016/j.ensm.2018.07.014
摘要

Developing high-energy rechargeable lithium-ion batteries (LIBs) is vital to the substantial development of electric vehicles and portable electronic devices. The limited specific capacity of the state-of-the-art cathode and anode materials is the biggest obstacle to high-energy LIBs. With regard to anode materials, Si has been regarded as one of the most promising next-generation anodes due to its substantially higher capacity (~ 4200 mA h g−1 for Li4.4Si) than traditional graphite anode (~ 372 mA h g−1), low operation potential, high abundance, and environmental friendliness. Several challenges need to be addressed, however, to make Si-based anodes commercially available, including such drawbacks as the tremendous volume variation during the discharge/charge process, unstable solid electrolyte interphase films, and poor electrical conductivity, which significantly restrict its practical application. In this review, we summarize the recent progress on Si-based anode materials from both the fundamental science point of view and the industrial perspective. From fundamental research to industrial application, the Si-based shell-containing nanostructures (core/shell and yolk/shell) and Si/graphite-based composites (Si/carbon and SiOx/carbon) are mainly covered to illustrate how these designs could solve the challenges of Si-based anodes. In addition, research progress on binders, electrolytes, and electrode additives towards enhanced electrochemical performance of Si-based anodes is also described. Finally, the remaining challenges and perspectives on the rational design of Si-based anode materials to realize commercialization are discussed and proposed.
最长约 10秒,即可获得该文献文件

科研通智能强力驱动
Strongly Powered by AbleSci AI
更新
大幅提高文件上传限制,最高150M (2024-4-1)

科研通是完全免费的文献互助平台,具备全网最快的应助速度,最高的求助完成率。 对每一个文献求助,科研通都将尽心尽力,给求助人一个满意的交代。
实时播报
Finit发布了新的文献求助10
刚刚
时光里完成签到,获得积分10
1秒前
篇篇高分发布了新的文献求助10
2秒前
ddj完成签到 ,获得积分10
3秒前
6秒前
笑点低梦露完成签到,获得积分10
8秒前
8秒前
YUMI发布了新的文献求助10
9秒前
大鸭完成签到,获得积分10
10秒前
RJH发布了新的文献求助10
11秒前
13秒前
13秒前
14秒前
研友_Ze0vBn完成签到,获得积分10
15秒前
宋志远发布了新的文献求助10
18秒前
失眠无声完成签到,获得积分10
18秒前
拜拜拜仁完成签到,获得积分10
18秒前
monere应助鹏826采纳,获得10
19秒前
田様应助josephina采纳,获得10
19秒前
VDC完成签到,获得积分0
20秒前
21秒前
冷傲的道罡完成签到,获得积分10
21秒前
wangzai111完成签到,获得积分10
22秒前
zcj发布了新的文献求助100
23秒前
25秒前
长情篮球发布了新的文献求助10
25秒前
27秒前
科研通AI2S应助Kvolu29采纳,获得10
27秒前
Jerry20184发布了新的文献求助10
28秒前
慕容松完成签到,获得积分10
28秒前
SciGPT应助LLL采纳,获得10
29秒前
30秒前
moralz发布了新的文献求助30
32秒前
33秒前
Joe完成签到,获得积分10
33秒前
33秒前
一碗鱼完成签到,获得积分10
34秒前
宋志远完成签到,获得积分10
34秒前
嗯好22222完成签到 ,获得积分10
34秒前
genomed应助梁晓玲采纳,获得10
34秒前
高分求助中
The late Devonian Standard Conodont Zonation 2000
The Lali Section: An Excellent Reference Section for Upper - Devonian in South China 1500
Nickel superalloy market size, share, growth, trends, and forecast 2023-2030 1000
Smart but Scattered: The Revolutionary Executive Skills Approach to Helping Kids Reach Their Potential (第二版) 1000
Mantiden: Faszinierende Lauerjäger Faszinierende Lauerjäger 800
PraxisRatgeber: Mantiden: Faszinierende Lauerjäger 800
A new species of Coccus (Homoptera: Coccoidea) from Malawi 500
热门求助领域 (近24小时)
化学 医学 生物 材料科学 工程类 有机化学 生物化学 物理 内科学 纳米技术 计算机科学 化学工程 复合材料 基因 遗传学 催化作用 物理化学 免疫学 量子力学 细胞生物学
热门帖子
关注 科研通微信公众号,转发送积分 3245829
求助须知:如何正确求助?哪些是违规求助? 2889464
关于积分的说明 8258504
捐赠科研通 2557814
什么是DOI,文献DOI怎么找? 1386661
科研通“疑难数据库(出版商)”最低求助积分说明 650327
邀请新用户注册赠送积分活动 626685