零价铁
沸石
化学
水溶液
氨
吸附
离子交换
氮气
无机化学
复合数
化学工程
核化学
催化作用
离子
材料科学
有机化学
工程类
复合材料
作者
Osama Eljamal,Ramadan Eljamal,Ibrahim Maamoun,Ahmed M.E. Khalil,Tamer Shubair,Omar Falyouna,Yuji Sugihara
出处
期刊:Chemosphere
[Elsevier]
日期:2022-01-01
卷期号:287: 131990-131990
被引量:80
标识
DOI:10.1016/j.chemosphere.2021.131990
摘要
The aim of the present study is developing a magnetic nanoscale zero-valent iron/zeolite (nZVI/Z) composite towards the efficient removal of ammonia-nitrogen (NH4+-N) from aqueous solutions. Series of batch experiments were conducted to investigate the effect of different factors on the removal efficiency, including pH effect, aerobic/anaerobic, NH4+-N initial concentration, and temperature. The mixing mass ratio of nZVI/Z was optimized to reach the optimal ratio (0.25 g nZVI: 0.75 g zeolite), corresponding to the best removal efficiency of 85.7% after 120 min of reaction. Results revealed that nZVI/Z is efficient for NH4+-N removal from water at a wide pH range (3.0–10.0), with superiority to the neutral conditions. Moreover, aerobic ambient and normal temperature of 25 °C were the optimal conditions for the removal process of NH4+-N. Removal mechanisms involved electrostatic attraction, ion exchange, and adsorption. Generally, nZVI/Z has great potential towards the practical applications of NH4+-N removal from water.
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