光催化
石墨烯
甲醇
氧化物
材料科学
催化作用
可见光谱
二氧化碳
化学工程
能量转换
纳米技术
化学
有机化学
光电子学
物理
工程类
冶金
热力学
作者
Hsin-Cheng Hsu,Indrajit Shown,Hsieh-Yu Wei,Yu-Chung Chang,He‐Yun Du,Yan‐Gu Lin,Chi-Ang Tseng,Chen‐Hao Wang,Li‐Chyong Chen,Yu‐Chuan Lin,Kuei‐Hsien Chen
出处
期刊:Nanoscale
[The Royal Society of Chemistry]
日期:2012-10-26
卷期号:5 (1): 262-268
被引量:439
摘要
Photocatalytic conversion of carbon dioxide (CO(2)) to hydrocarbons such as methanol makes possible simultaneous solar energy harvesting and CO(2) reduction, two birds with one stone for the energy and environmental issues. This work describes a high photocatalytic conversion of CO(2) to methanol using graphene oxides (GOs) as a promising photocatalyst. The modified Hummer's method has been applied to synthesize the GO based photocatalyst for the enhanced catalytic activity. The photocatalytic CO(2) to methanol conversion rate on modified graphene oxide (GO-3) is 0.172 μmol g cat(-1) h(-1) under visible light, which is six-fold higher than the pure TiO(2).
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