材料科学
聚苯胺
纳米纤维
摩擦电效应
吸附
相对湿度
纳米技术
纳米发生器
响应时间
化学工程
湿度
聚苯胺纳米纤维
聚合物
复合材料
聚合
化学
计算机科学
有机化学
压电
工程类
计算机图形学(图像)
物理
热力学
作者
Si Wang,Bohao Liu,Zaihua Duan,Qiuni Zhao,Yajie Zhang,Guangzhong Xie,Yadong Jiang,Shaorong Li,Huiling Tai
标识
DOI:10.1016/j.snb.2020.128923
摘要
As a new member of the MXene family, two dimensional (2D) niobium carbide MXene (Nb2CTx) holds a promising potential in gas detection due to the abundant surface terminated groups and large specific surface area. In this work, a selective NH3 sensor based on polyaniline (PANI) nanofibers-supported Nb2CTx nanosheets (Nb2CTx/PANI) directly driven by a facile triboelectric nanogenerator (TENG) is proposed to provide a possible method for enhancing the NH3-sensing response. In addition, the gas sensing properties have been optimized by regulating different spray volumes of Nb2CTx nanosheets. Test results demonstrate that the NH3-sensing response and the response speed of the Nb2CTx/PANI-2 sensor have been evidently improved, indicating a good linear response toward a wide sensing range of 1–100 ppm NH3 at room temperature (∼25℃) under 87.1 % relative humidity (RH). Moreover, the influence of high humidity on gas sensing response of the Nb2CTx/PANI-2 sensor has been efficiently reduced due to the occupied active sites for water adsorption caused by intermolecular hydrogen bonds between PANI and Nb2CTx. Finally, mechanism of the enhanced gas sensing properties has been further investigated, which should be mainly attributed to the gas sensing improvement effect of p-n junction. This work is expected to offer a useful reference for the development of high-performance Nb2CTx/polymer-based gas sensors.
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