Redesigning Natural Materials for Energy, Water, Environment, and Devices

The United Nations Framework Convention on Climate Change (UNFCCC) acknowledges that global cooperation is paramount to mitigate climate change and further warming. The global community is committed to renewable energy and natural materials to tackle this challenge for all humankind. The widespread use of natural materials is embraced as one such action to reach net-zero carbon emissions. Given the hierarchical framework and earth abundance, cellulose-based materials extend their negative carbon benefits to our daily products and accelerate our pace toward carbon neutrality. Here, we present an overview of recent developments of cellulose-based materials in upsurging applications in radiative cooling, thermal insulation, nanofluidics, and wearable devices. We also highlight various modifications and functionalized processes that transform massive amounts of cellulose into green products. The prosperous development of functionalized cellulose materials aligns with a circular economy. Expedited interdisciplinary fundamental investigations are expected to make fibrillated cellulose penetrate more into carbon downdraw at speed and scale.