First Assessment of NOx Sources at a Regional Background Site in North China Using Isotopic Analysis Linked with Modeling

环境科学 同位素分析 中国 考古 海洋学 地质学 地理
作者
Zheng Zong,Xiaoping Wang,Chongguo Tian,Yingjun Chen,Yunting Fang,Fan Zhang,Cheng Li,Jianzhong Sun,Jun Li,Gan Zhang
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:51 (11): 5923-5931 被引量:178
标识
DOI:10.1021/acs.est.6b06316
摘要

Nitrogen oxides (NOx, including NO and NO2) play an important role in the formation of atmospheric particles. Thus, NOx emission reduction is critical for improving air quality, especially in severely air-polluted regions (e.g., North China). In this study, the source of NOx was investigated by the isotopic composition (δ15N) of particulate nitrate (p-NO3-) at Beihuangcheng Island (BH), a regional background site in North China. It was found that the δ15N-NO3- (n = 120) values varied between -1.7‰ and +24.0‰ and the δ18O-NO3- values ranged from 49.4‰ to 103.9‰. On the basis of the Bayesian mixing model, 27.78 ± 8.89%, 36.53 ± 6.66%, 22.01 ± 6.92%, and 13.68 ± 3.16% of annual NOx could be attributed to biomass burning, coal combustion, mobile sources, and biogenic soil emissions, respectively. Seasonally, the four sources were similar in spring and fall. Biogenic soil emissions were augmented in summer in association with the hot and rainy weather. Coal combustion increased significantly in winter with other sources showing an obvious decline. This study confirmed that isotope-modeling by δ15N-NO3- is a promising tool for partitioning NOx sources and provides guidance to policymakers with regard to options for NOx reduction in North China.
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