材料科学
金属锂
固态
锂(药物)
聚合物电解质
聚合物
电解质
快离子导体
金属
电导率
灵活性(工程)
金属有机骨架
纳米技术
工程物理
离子电导率
物理化学
电极
复合材料
冶金
吸附
化学
内分泌学
工程类
统计
医学
数学
作者
Song Duan,Lanting Qian,Yun Zheng,Yanfei Zhu,Fei Liu,Dong Li,Wei Yan,Jiujun Zhang
标识
DOI:10.1002/adma.202314120
摘要
Solid polymer electrolytes (SPEs) for lithium metal batteries have garnered considerable interests owing to their low cost, flexibility, lightweight, and favorable interfacial compatibility with battery electrodes. Their soft mechanical nature compared to solid inorganic electrolytes give them a large advantage to be used in low pressure solid-state lithium metal batteries, which can avoid the cost and weight of the pressure cages. However, the application of SPEs is hindered by their relatively low ionic conductivity. In addressing this limitation, enormous efforts are devoted to the experimental investigation and theoretical calculations/simulation of new polymer classes. Recently, metal-organic frameworks (MOFs) have been shown to be effective in enhancing ion transport in SPEs. However, the mechanisms in enhancing Li
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