Flexible Triboelectric Tactile Sensor Based on a Robust MXene/Leather Film for Human–Machine Interaction

With the rapid development of Internet of Things (IoT) technology in recent years, self-actuated sensor systems without an external power supply such as flexible triboelectric nanogenerator (TENG)-based strain sensors have received wide attention due to their simple structure and self-powered active sensing properties. However, to satisfy the practical applications of human wearable biointegration, flexible TENGs impose higher requirements for establishing a balance between material flexibility and good electrical properties. In this work, the strength of the MXene/substrate interface was greatly improved by utilizing leather with a unique surface structure as the substrate material, resulting in a mechanically strong and electrically conductive MXene film. Due to the natural fiber structure of the leather surface, the surface of the MXene film with a rough structure was obtained, which improved the electrical output performance of the TENG. The electrode output voltage of MXene film on leather based on single-electrode TENG can reach 199.56 V and the maximum output power density can reach 0.469 mW/cm2. Combined with laser-assisted technology, the efficient array preparation of MXene and graphene was achieved and applied to various human-machine interface (HMI) applications.