Carbonized Polymer Dots: A Brand New Perspective to Recognize Luminescent Carbon-Based Nanomaterials

Carbon dots (CDs), as emerging luminescent nanomaterials, possess excellent but complex properties, bringing about extensive attention and a lot of controversy. In this Perspective, we put forward the concept of "carbonized polymer dots" and emphasize the important role of polymerization and carbonization during the formation of CDs. We explore the common characters and clarify the complicated relationship of CDs, based on the reasonable classification of graphene quantum dots, carbon quantum dots, and carbonized polymer dots. Moreover, different perspectives are provided for comprehensive analysis about the essence of CDs, including quantum dots, molecules, and polymers. The photoluminescence mechanism has been classified into molecule state, carbon core state, surface/edge state, and cross-link enhanced emission effect for further understanding of complicated phenomena.