Magnetic Skyrmions above Room Temperature in a van der Waals Ferromagnet Fe3GaTe2

Abstract 2D van der Waals (vdW) ferromagnetic crystals are a promising platform for innovative spintronic devices based on magnetic skyrmions, thanks to their high flexibility and atomic thickness stability. However, room‐temperature skyrmion‐hosting vdW materials are scarce, which poses a challenge for practical applications. In this study, a chemical vapor transport (CVT) approach is employed to synthesize Fe 3 GaTe 2 crystals and room‐temperature Néel skyrmions are observed in Fe 3 GaTe 2 nanoflakes above 58 nm in thickness through in situ Lorentz transmission electron microscopy (L‐TEM). Upon an optimized field cooling procedure, zero‐field hexagonal skyrmion lattices are successfully generated in nanoflakes with an extended thickness range (30–180 nm). Significantly, these skyrmion lattices remain stable up to 355 K, setting a new record for the highest temperature at which skyrmions can be hosted. The research establishes Fe 3 GaTe 2 as an emerging above‐room‐temperature skyrmion‐hosting vdW material, holding great promise for future spintronics.