Sorption-based atmospheric water harvesting for continuous water production in the built environment: Assessment of water yield and quality

环境科学 水质 吸附 相对湿度 产量(工程) 溶解有机碳 湿度 水处理 环境工程 原水 环境化学 制浆造纸工业 化学 吸附 气象学 物理 工程类 生物 有机化学 冶金 材料科学 生态学
作者
Chao Zeng,Amin Mojiri,Jirapat Ananpattarachai,Alireza Farsad,Paul Westerhoff
出处
期刊:Water Research [Elsevier]
卷期号:265: 122227-122227 被引量:1
标识
DOI:10.1016/j.watres.2024.122227
摘要

Sorption-based atmospheric water harvesting (SAWH) is a promising solution for localized high-quality water production. Application of SAWH indoors offers dual benefits of on-site water generation and humidity control. This study evaluated the use of SAWH for water production in residential or office buildings, employing a portable zeolite-based SAWH device. Over the twelve-month testing period in the arid southwestern USA, the device achieved a median water yield of 3.6 L/day at a cost 30 % less than bottled water sold in the U.S. A mathematical model was developed for predicting water yield under different temperature and relative humidity (RH) conditions. Daily water yields were well fitted with the modified Langmuir model, with absolute humidity serving as the only prediction variable. Water extracted from a well-ventilated office building generally met the drinking water standards set by USEPA. However, elevated levels of dissolved organic carbon (DOC) were detected in the samples collected from the residential house (median = 32.6 mg/L), emphasizing the influence of human activities (e.g., cooking) on the emission of volatile and semi-volatile organic compounds in the air, which consequently reside in harvested water. Aldehydes and volatile fatty acids (formate, acetate) comprised roughly 50 % of the DOC found in the AWE water. A carbon fiber filter was not effective at removing these substances, highlighting the need for further research into effective treatment methods for DOC management before the safe use of AWE water. Overall, this study provides critical insights for the practical application of indoor SAWH as a decentralized source of high-quality water and emphasizes the need to identify and manage DOC for its safe use.

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