光催化
异质结
表面等离子共振
可见光谱
等离子体子
催化作用
降级(电信)
材料科学
吸收(声学)
光电子学
化学工程
纳米颗粒
纳米技术
化学
计算机科学
有机化学
电信
工程类
复合材料
作者
Wei Zhao,Mengru Yan,Xinran Yang,Xiaojun Zeng,Yantong Chen,Benlin Dai,Xiaozhong Chu,Xuekun Hong,Feihu Mu,Shijie Li,Dennis Y.C. Leung
标识
DOI:10.1016/j.seppur.2022.122896
摘要
Environmental pollution caused by the overusage and uncontrolled discharge of antibiotics such as amoxicillin will endanger public health and ecosystems. Herein, a novel Ag/MIL-68(In)-NH2/Bi4O7 plasmonic heterojunction has been successfully prepared through a two-step route followed by photoreduction for environmentally friendly photocatalytic amoxicillin degradation. Ag/MIL-68(In)-NH2/Bi4O7 displayed the most efficient photocatalytic performance, which was 3.7 and 3.2 times that of Bi4O7 and MIL-68(In)-NH2, respectively. The superior photocatalytic activity was directly linked to its large surface area and localized surface plasmon resonance (LSPR) effect, which provides more active sites and effectively promotes visible light absorption. Moreover, the degradation path of amoxicillin was explored in detail by combining Gaussian software calculation with liquid chromatography-mass spectrometry (LC-MS) analysis. Finally, a series of characterizations and simulations were carried out to demonstrate the S-scheme photocatalytic mechanism.
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