Metal–organic frameworks for the generation of reactive oxygen species

活性氧 纳米技术 金属有机骨架 氧化应激 材料科学 有机分子 催化作用 有机合成 化学 分子 有机化学 生物化学 吸附
作者
Hudson A. Bicalho,Victor Quezada‐Novoa,Ashlee J. Howarth
出处
期刊:Chemical physics reviews [American Institute of Physics]
卷期号:2 (4) 被引量:13
标识
DOI:10.1063/5.0060141
摘要

Reactive oxygen species (ROS) are highly reactive molecules derived from oxygen, which are naturally generated and play essential roles in biological processes. At the same time, ROS are the basis of advanced oxidation processes (AOPs), which can be used for multiple applications of industrial interest, including water treatment and organic synthesis. Additionally, anti-cancer therapies that involve the targeted production of ROS in cancerous cells have shown promising results in vitro and in vivo by promoting oxidative stress and, hence, cell death. However, up to this day, the development of catalysts and systems that are, at the same time, easily synthesized, low-cost, nontoxic, and highly effective remains a challenge. With that in mind, metal–organic frameworks (MOFs), a relatively new class of coordination polymers, may display all these characteristics and many others, including tunable structure, extensive porosity, and high surface areas. Because of that, the design and synthesis of MOFs and MOF-based materials for the generation of ROS has garnered attention in recent years. In this review, we summarize recent advances in the development and use of MOFs or MOF-based materials as catalysts in AOPs and biological systems through the generation of ROS, shining light on promising results and future research directions.
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