Air Quality Data Approach for Defining Wildfire Influence: Impacts on PM2.5, NO2, CO, and O3 in Western Canadian Cities

体裂 空气质量指数 环境科学 拦截 气象学 污染物 空气污染 弹道 大气科学 空气污染物 气候变化 气候学 气溶胶 地理 生态学 物理 生物 地质学 有机化学 化学 天文
作者
Stephanie R. Schneider,Kristyn Lee,Guadalupe Santos,Jonathan P. D. Abbatt
出处
期刊:Environmental Science & Technology [American Chemical Society]
卷期号:55 (20): 13709-13717 被引量:34
标识
DOI:10.1021/acs.est.1c04042
摘要

As the climate warms, it is recognized that wildfires are increasing in size and frequency. The negative effects of wildfires on air quality are well documented, especially on commonly monitored atmospheric pollutants such as PM2.5, NO2, CO, and O3. However, it is not clear how frequently wildfires influence urban air quality and the size of that influence relative to traffic and industrial pollutants. To understand the impact of wildfires on air quality, we have established an automated method to identify wildfire-influenced ambient air measurements. The trajectory-fire interception method (TFIM) compares hybrid single-particle Lagrangian integrated trajectory (HYSPLIT) back-trajectories from an air quality monitoring station to satellite imagery of fire "hot-spots" to determine the number of trajectory-fire interceptions that occur. From the number of interceptions and local PM2.5 measurements, we have defined a wildfire-influenced period to occur if the interception count is ≥20. TFIM wildfire identification compares favorably with Environment and Climate Change Canada's smoke forecast, FireWork, and with the BlueSky trajectory-based forecast. Using TFIM, we studied the impact of wildfire-influenced periods on PM2.5, NO2, CO, and O3 from 2001 to 2019 in Western Canadian urban areas. We show that wildfire-influenced periods have elevated concentrations of PM2.5, NO2, and CO but not O3. We show that a decreasing urban baseline of CO and NO2 over time results in a relatively greater impact of wildfires on these pollutants, which emphasizes the changing relative importance of wildfires on air quality.
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