Advanced Anode Materials for Rechargeable Sodium-Ion Batteries

阳极 材料科学 纳米技术 电化学 锂(药物) 储能 杂原子 电极 化学 戒指(化学) 有机化学 功率(物理) 物理化学 内分泌学 物理 医学 量子力学
作者
Shuangyan Qiao,Qianwen Zhou,Meng Ma,Huan Liu,Shi Xue Dou,Shaokun Chong
出处
期刊:ACS Nano [American Chemical Society]
卷期号:17 (12): 11220-11252 被引量:303
标识
DOI:10.1021/acsnano.3c02892
摘要

Rechargeable sodium-ion batteries (SIBs) have been considered as promising energy storage devices owing to the similar "rocking chair" working mechanism as lithium-ion batteries and abundant and low-cost sodium resource. However, the large ionic radius of the Na-ion (1.07 Å) brings a key scientific challenge, restricting the development of electrode materials for SIBs, and the infeasibility of graphite and silicon in reversible Na-ion storage further promotes the investigation of advanced anode materials. Currently, the key issues facing anode materials include sluggish electrochemical kinetics and a large volume expansion. Despite these challenges, substantial conceptual and experimental progress has been made in the past. Herein, we present a brief review of the recent development of intercalation, conversion, alloying, conversion-alloying, and organic anode materials for SIBs. Starting from the historical research progress of anode electrodes, the detailed Na-ion storage mechanism is analyzed. Various optimization strategies to improve the electrochemical properties of anodes are summarized, including phase state adjustment, defect introduction, molecular engineering, nanostructure design, composite construction, heterostructure synthesis, and heteroatom doping. Furthermore, the associated merits and drawbacks of each class of material are outlined, and the challenges and possible future directions for high-performance anode materials are discussed.
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