材料科学
尖晶石
催化作用
铱
氧化物
溶解
析氧
无机化学
物理化学
电化学
化学
冶金
电极
生物化学
作者
Ashwani Kumar,Marcos Gil‐Sepulcre,Jinsun Lee,Viet Q. Bui,Yue Wang,Olaf Rüdiger,Min Gyu Kim,Serena DeBeer,Harun Tüysüz
标识
DOI:10.1002/adma.202401648
摘要
Exploring single-atom-catalysts for the acidic oxygen evolution reaction (OER) is of paramount importance for cost-effective hydrogen production via acidic water electrolyzers. However, the limited durability of most single-atom-catalysts and Ir/Ru-based oxides under harsh acidic OER conditions, primarily attributed to excessive lattice oxygen participation resulting in metal-leaching and structural collapse, hinders their practical application. Herein, an innovative strategy is developed to fabricate short-range Ir single-atom-ensembles (Ir
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