Giant broadband spin-selective asymmetric transmission and wavefront shaping in transition-metal-dichalcogenide-based chiral metasurfaces

Multidimensional spin-selective manipulation of optical waves is crucial for various intriguing applications in modern nanophotonics, such as quantum-information processing and chiral sensing and imaging. In this work, we observed giant broadband asymmetric transmission of circularly polarized waves and spin-preserving reflection, together with near-unity transmission circular dichroism, in a planar chiral metasurface composed of high-index transition-metal-dichalcogenide nanoantennas with large material anisotropy. The perpendicular and parallel electric and magnetic dipole moments excited in the nanoantennas under circularly polarized waves are explored to account for the asymmetric transmission and optical chirality. Combined with the Pancharatnam–Berry phase, we achieved the wavefront manipulation for transmitted circularly polarized waves with an efficiency approaching 91.5% and spin-selective focusing of an incident light via a metasurface metalens. Our work will pave the way for studying the multidimensional manipulation of optical spins through engineering transition-metal-dichalcogenide-based metasurfaces.