Quantification of greenhouse gas emission from wastewater treatment plants

温室气体 污水处理 曝气 甲烷 二氧化碳 厌氧消化 一氧化二氮 环境科学 生物固体 废水 环境工程 活性污泥 化学 废物管理 环境化学 生态学 工程类 生物 有机化学
作者
Ruolin Bai,Lei Jin,Shu-Yu Sun,Yang Cheng,Yi Wei
出处
期刊:Greenhouse Gases-Science and Technology [Wiley]
卷期号:12 (5): 587-601 被引量:7
标识
DOI:10.1002/ghg.2171
摘要

Abstract In this study, a new quantitative approach of greenhouse gas (GHG) emissions from wastewater treatment plants (WWTPs) is established. It is developed based on three categories of WWPTs: (1) energy and chemical consumption; (2) final disposal of biosolids; and direct GHG emission from treatment processes, which is helpful to better estimate the GHG emission pathways. The developed approach can provide actual results of GHG emission in terms of carbon dioxide (CO 2 ), nitrous oxide (N 2 O), and methane (CH 4 ) from wastewater treatment process. Then, this method is applied to a municipal WWPT, where the GHG emission from the processes of final treatment, biological treatment, and anaerobic digestion, at the southside of Guelph city in Canada. The results show that there are 6743.8 CO 2 eq.kg/day of CO 2 and 1924.48 CO 2 eq.kg/day of N 2 O emissions from aeration tank/activated sludge system. The biological treatment and anaerobic digestion release 74177.58 CO 2 eq.kg/day of CH 4 , 7258.5 CO 2 eq.kg/day of CO 2 , and 59022.6 CO 2 eq.kg/day of CH 4 , 3493.24 CO 2 eq.kg/day of CO 2 . If the methane, which discharged from biological treatment and anaerobic digestion, is captured and burned for energy regeneration, then it can produce 12937.9 CO 2 eq.kg/day of CO 2 . The total amount of GHG indicates that about 80% GHG is emitted from the final disposal field while 9% and 11% GHG is emitted from biological treatment and anaerobic digestion, respectively. Therefore, based on the calculated results, engineers can put forward suggestions to optimize operation conditions to reduce greenhouse gas emissions. © 2022 Society of Chemical Industry and John Wiley & Sons, Ltd.
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