材料科学
纳米材料
纳米线
宽带
各向异性
双折射
纳米技术
光电子学
波长
纳米晶
光学
物理
作者
Jiawei Lv,Ke Hou,Defang Ding,Dawei Wang,Bing Han,Xiaoqing Gao,Man Zhao,Lin Shi,Jun Guo,Yonglong Zheng,Xi Zhang,Chenguang Lu,Ling Huang,Wei Huang,Zhiyong Tang
标识
DOI:10.1002/anie.201701512
摘要
Abstract An ultrastrong and broadband chiroptical response is key but remains challenging for many device applications. A simple and cost‐effective bottom‐up method is introduced to fabricate large‐area long‐range ordered chiral ultrathin films with the Langmuir–Schaeffer technique using gold nanowires as building blocks. Significantly, as‐prepared ultrathin films display giant optical activity across a broad wavelength range covering visible and near infrared regions with an anisotropic factor of up to 0.285, which is the record value for bottom‐up techniques. Detailed experimental result and theoretical analysis disclose that such remarkable optical activity originates from birefringence and dichroism of the well‐aligned Au nanowire layers in the ultrathin films. The universality of this facile strategy for constructing chiral ultrathin films is further demonstrated with many other one‐dimensional nanomaterials.
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