阳极
催化作用
直接甲醇燃料电池
甲醇燃料
材料科学
阴极
电极
功率密度
使用寿命
电流密度
温度梯度
化学工程
复合材料
功率(物理)
化学
电气工程
工程类
有机化学
物理
物理化学
量子力学
作者
Zhixin Chang,Jiajia Zhang,Weiqi Zhang,Huaneng Su,Lei Xing,Qiang Ma,Hong Zhang,Qian Xu
出处
期刊:Processes
[MDPI AG]
日期:2021-10-08
卷期号:9 (10): 1787-1787
被引量:3
摘要
Direct methanol fuel cells (DMFCs) offer high energy density, simple liquid fuel storage, and the ability to operate at ambient temperature. They may be used in a variety of portable mobile power supplies, small civilian power supplies, and automotive power supplies. However, in the process of electrochemical reaction inside a DMFC, because the reactants and products are distributed unevenly, the in-plane concentration of reactants and reaction rate are different; thus, the current density generated in the active area shows a high degree of non-uniformity. The high local current density can easily lead to the acceleration of DMFC aging. As a result, the operating cost of the DMFC is increased and the service life is shortened, which limits the commercial application of DMFCs. In this work, we develop an in-plane gradient loading catalyst. The loading on both the anode and cathode catalysts was lower near the inlet and higher close to the outlet. The experimental results of the single-cell test show that the performance of the gradient loading catalyst electrode was enhanced by up to 19.8% compared with the uniform loading catalyst at 60 °C for the same catalyst loading, especially under high current densities. In addition, the catalyst utilization was improved for the gradient loading catalyst electrode. Hence, the proposed approach shows potential for reducing the cost and increasing the service life of DMFCs.
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