材料科学
电子设备和系统的热管理
制作
石墨烯
二硫化钼
热的
可见光谱
纳米技术
光电子学
复合材料
机械工程
物理
工程类
病理
气象学
医学
替代医学
作者
Kerui Li,Ting‐Hsiang Chang,Zhipeng Li,Haitao Yang,Fanfan Fu,Tingting Li,John S. Ho,Po‐Yen Chen
标识
DOI:10.1002/aenm.201901687
摘要
Abstract 2D materials are of particular interest in light‐to‐heat conversion, yet challenges remain in developing a facile method to suppress their light reflection. Herein, inspired by the black scales of Bitis rhinoceros , a generalized approach via sequential thermal actuations to construct biomimetic 2D‐material nanocoatings, including Ti 3 C 2 T x MXene, reduced graphene oxide (rGO), and molybdenum disulfide (MoS 2 ) is designed. The hierarchical MXene nanocoatings result in broadband light absorption (up to 93.2%), theoretically validated by optical modeling and simulations, and realize improved light‐to‐heat performance (equilibrium temperature of 65.4 °C under one‐sun illumination). With efficient light‐to‐heat conversion, the bioinspired MXene nanocoatings are next incorporated into solar steam‐generation devices and stretchable solar/electric dual‐heaters. The MXene steam‐generation devices require much lower solar‐thermal material loading (0.32 mg cm −2 ) and still guarantee high steam‐generation performance (1.33 kg m −2 h −1 ) compared with other state‐of‐the‐art devices. Additionally, the mechanically deformed MXene structures enable the fabrication of stretchable and wearable heaters dual‐powered by sunlight and electricity, which are reversibly stretched and heated above 100 °C. This simple fabrication process with effective utilization of active materials promises its practical application value for multiple solar–thermal technologies.
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