Chirality induced spin selectivity in chiral hybrid organic–inorganic perovskites

自旋电子学 手性(物理) 材料科学 自旋(空气动力学) 圆二色性 纳米技术 光致发光 选择性 化学物理 化学 铁磁性 凝聚态物理 光电子学 物理 对称性破坏 结晶学 有机化学 量子力学 手征对称破缺 Nambu–Jona Lasinio模型 热力学 催化作用
作者
Jingying Wang,Baorui Mao,Z. Valy Vardeny
出处
期刊:Journal of Chemical Physics [American Institute of Physics]
卷期号:159 (9) 被引量:9
标识
DOI:10.1063/5.0160032
摘要

Chiral materials exhibit many interesting physical properties including circular dichroism, circularly polarized photoluminescence, and spin selectivity. Since its discovery, chirality-induced spin selectivity (CISS) has been demonstrated in many chiral material systems, which indicates promising applications in spintronic devices. Thus, searching for compounds that possess both sizable chirality and excellent spin transport properties is in order. Hybrid organic-inorganic perovskites have attracted intensive research interest due to their long carrier lifetime, high carrier mobility, chemically tunable electronic properties, and long spin lifetime, which make this emerging class of semiconductors promising candidate for spintronics. Moreover, hybrid perovskites integrate inorganic octahedral framework and organic ligands, which may introduce chirality into the materials, especially in quasi-two-dimensional structures. Recently, CISS has been observed in 2D chiral hybrid perovskites, showing the spin filtering effect. Studies of CISS in chiral hybrid perovskites not only help deepen our understanding of CISS mechanism but also shed new light on designing novel spintronic devices. In this review, we summarize the state-of-the-art studies of CISS effect in 2D chiral hybrid organic-inorganic perovskites system. We also discuss the remaining challenges and research opportunities of employing CISS in next-generation spintronic devices.
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