臭氧
过氧化氢
电晕放电
电极
相(物质)
放电
化学
分析化学(期刊)
材料科学
非热等离子体
氢
化学工程
等离子体
色谱法
有机化学
物理化学
工程类
物理
量子力学
作者
Petr Lukeš,A.T. Appleton,Bruce R. Locke
出处
期刊:IEEE Transactions on Industry Applications
[Institute of Electrical and Electronics Engineers]
日期:2004-01-01
卷期号:40 (1): 60-67
被引量:212
标识
DOI:10.1109/tia.2003.821799
摘要
Ozone in the gas phase and hydrogen peroxide in the liquid phase were simultaneously formed in hybrid electrical discharge reactors, known as the hybrid-series and hybrid-parallel reactors, which utilize both gas phase nonthermal plasma formed above the water surface and direct liquid phase corona-like discharge in the water. In the series configuration the high voltage needle-point electrode is submerged and the ground electrode is placed in the gas phase above the water surface. The parallel configuration employs a high voltage electrode in the gas phase and a high voltage needle-point electrode in the liquid phase with the ground electrode placed at the gas-liquid interface. In both hybrid reactors the gas phase concentration of ozone reached a power-dependent steady state, whereas the hybrid-parallel reactor produced a substantially larger amount of ozone than the hybrid series. Hydrogen peroxide was produced in both hybrid reactors at a similar rate to that of a single-phase liquid electrical discharge reactor. The resulting concentration of H/sub 2/O/sub 2/ in the hybrid reactors, however, depended on the pH of the solution and the gas phase ozone concentration since H/sub 2/O/sub 2/ was decomposed by dissolved ozone at high pH.
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