光催化
异质结
降级(电信)
可见光谱
材料科学
纳米复合材料
化学工程
氧化还原
载流子
纳米技术
复合数
光化学
催化作用
光电子学
化学
复合材料
计算机科学
有机化学
工程类
冶金
电信
作者
Feng Guo,Weilong Shi,Mingyang Li,Yu Shi,Huabing Wen
标识
DOI:10.1016/j.seppur.2018.08.055
摘要
Photocatalysis is one of the most promising technologies owing to its great potential to relieve energy and environmental issues. Constructing Z-scheme heterojunction photocatalyst with strong redox ability to make for enhanced light absorption and efficient charge separation is extremely attractive but still underdeveloped. Herein, Z-scheme heterojunction of CuInS2/g-C3N4 with a “sheet-on-sheet” hierarchical structure showing enhanced photocatalytic performance for the tetracycline (TC) degradation under visible-light irradiation has been developed. This 2D/2D hierarchical structure of CuInS2/g-C3N4 composite not only enlarges the contact region in the heterojunction interface but also provides more active reaction sites, as demonstrated by the TEM and BET analyses. Particularly, 50 wt% CuInS2/g-C3N4 heterojunction shows the highest photocatalytic activity (20 mg/L; 83.7% degradation within 60 min), which the apparent rate constant is 15 and 11 times higher than that of pure g-C3N4 and CuInS2 nanosheets, respectively. The remarkably enhanced photocatalytic activity mainly derives from the synergistic effect between CuInS2 and g-C3N4, thereby promoting the charge separation during the photocatalytic reaction. This work is expected to provide a design idea to construct multifunctional 2D/2D nanocomposites for photocatalytic applications.
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