Incorporating Metal Precursors towards a Library of High-resolution Metal Parts by Stereolithography

立体光刻 金属 高分辨率 材料科学 工程类 纳米技术 冶金 复合材料 地质学 遥感
作者
Yuemeng Li,Chen Li,Xin Zhang,Yanqing Wang,Yonghao Tan,Shuai Chang,Zhe Chen,Gangwen Fu,Zongkui Kou,Stefan Adams,Xi Xu,Jun Ding
出处
期刊:Applied Materials Today [Elsevier BV]
卷期号:29: 101553-101553 被引量:15
标识
DOI:10.1016/j.apmt.2022.101553
摘要

• A new metal AM method using DLP printed metal precursors realizes metal/alloy components with fine feature size, large dimension, robust structure, and promising properties. • DLP was leveraged to create a robust structure with high resolution. • As-fabricated 3D printed metals have been demonstrated to possess excellent electric and mechanical properties with low surface roughness. Additive manufacturing (AM) of three-dimensional (3D) metals with intricate fine features and complex geometry at the macro- and micro- scale for energy generation and storage has attracted great interest recently. Fabrication of metals using state-of-art powder-based AM technology with high resolution and tunable microstructure remains a challenge. In this work, a new method for achieving sophisticated metallic structure via the digital light process (DLP) of metal precursors containing photo-resin followed by thermal heating and chemical reduction process is presented. Thermal decomposition of 3D-printed metal compound and chemical reduction makes it promising to synthesize a morphology-tunable and geometrically complex metal, alloy, metal oxide, or multi-material component. Two potential applications of 3D-printed copper using this method are demonstrated in the electrochemical field as oxygen evolution reaction (OER) catalyst support and current collector. NiFe hydroxide@3D-printed copper can drive a 100 mA/cm 2 stably with a low energy barrier in an alkaline solution. Galvanostatic cycling profile of DLP Copper/electrolyte/Li at current densities of 2 mA/cm 2 , 4 mA/cm 2 and 10 mA/cm 2 can be conducted stably for a capacity of 20 mA·h/cm 2 . This work is the first to realize metal-based printing with ultra-high resolution thorough photopolymerization.
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