Remarkably enhanced hydrogen evolution of g-C3N4 nanosheet under simulated sunlight via AgPt alloy co-catalyst with low amount of Pt

双金属片 光催化 催化作用 材料科学 制氢 纳米颗粒 化学工程 纳米片 合金 分解水 金属 光化学 纳米技术 化学 冶金 有机化学 工程类
作者
Ganghua Zhou,Longyun Zhang,Yu Xia,Weiqin Yin,Xingwang Zhu,Jianhua Hou,Shengsen Wang,Xin Ning,Xiaozhi Wang
出处
期刊:Journal of Cleaner Production [Elsevier BV]
卷期号:434: 139950-139950 被引量:19
标识
DOI:10.1016/j.jclepro.2023.139950
摘要

The development of low-cost co-catalysts matched with proper photocatalysts to enhance the photocatalytic hydrogen evolution performance is highly demanded. Herein, the AgPt bimetallic alloy nanoparticles with small amounts of Pt were decorated on g-C3N4 nanosheets (AP-CN) via the NaBH4 reduction method, which were further used as catalysts towards photocatalytic hydrogen evolution from water under AM1.5 irradiation. Compared to mono-metallic co-catalysts, bimetallic AgPt alloy nanoparticles exhibited excellent co-catalytic performance. The optimum AP-CN photocatalyst with 0.5 wt% Pt exhibited photocatalytic hydrogen evolution rate of 3507.89 μmol g−1·h−1, which even surpassed that of the commonly-used photocatalyst 1.0 wt% Pt in-situ photo-deposited on g-C3N4. Meanwhile, the AP-CN showed excellent photocatalytic activity and durability after four experimental cycles. The enhanced activity and stability could be attributed to the synergistic effect between plasmonic metal Ag and Pt, which promoted the transfer and separation of photoinduced charge carriers. Besides, the theoretical results based on DFT calculation also verified that AgPt alloys have better performance of desorbing hydrogen and adsorbing H atoms. This work provides a feasible idea for the development of inexpensive and efficient bimetallic co-catalysts for photocatalytic hydrogen production through water splitting.
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