Stretchable polymeric modulator for intracavity spectroscopic broadening of femtosecond optical parametric oscillators

We investigate stretching-induced microscopic deformations spatially distributed in a flexible plate of polydimethylsiloxane (PDMS) and their applications in the broadening of the output spectrum of a femtosecond optical parametric oscillator. The hologram of the stretched PDMS plate was used to evaluate indirectly the microscopic deformations. The experimental results show that these deformations exhibit weak scattering and diffraction of light and induce negligible cavity loss, ensuring practical applications of the PDMS plate as an intracavity device for lasers. In combination with the thickness reduction of the PDMS plate through stretching, the distributed deformations enable smooth tuning of the output spectrum.