水分
钙钛矿(结构)
材料科学
化学工程
环境科学
复合材料
工程类
作者
Yang Zhang,Chuanxiang Sheng,Pingyuan Yan,Zhifu Zhu,Yong Gan
标识
DOI:10.1016/j.mseb.2024.117423
摘要
This work applies comprehensively researches on the influence of water as an additive in precursor solution, and the moisture (65 % relative humidity) on the performance of Dion-Jacobson (DJ) perovskite [C6H4(CH2NH3)2] (CH2NH3)3Pb4I13 solar cells. The results indicate that 3 %−15 % (v/v) water as an additive has minor effect on the power conversion efficiency (PCE) of fresh prepared solar cells, but it can improve the resistance of device to humidity. More importantly, with an appropriate ratio of water additive and moister action time, the perovskite film shows a smoother surface, higher coverage, and better crystallinity, resulting in an optimal PCE of ∼ 8 %, compared to ∼ 1 % of fresh prepared one. Our results are helpful to understand the effect of water and moisture on DJ perovskite solar cells, may contributing to develop rational strategies to improve devices' stability under humidity ambient.
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