六价铬
罗丹明B
纳米复合材料
压电
催化作用
环境修复
材料科学
降级(电信)
纳米片
化学工程
异质结
纳米技术
铬
复合材料
化学
光电子学
冶金
电信
污染
工程类
生态学
生物
光催化
生物化学
计算机科学
作者
Hongjing Li,Yi Xiong,Yumin Wang,Wenmei Ma,Jiapeng Fang,Xu Li,Qing Han,Yong Liu,Chunqing He,Pengfei Fang
标识
DOI:10.1016/j.jcis.2021.11.070
摘要
Piezocatalysis, driven by mechanical energy and piezoelectric effect, is of great potential in addressing the environmental issues. In this work, a piezoelectric catalyst was fabricated by growing few-layer MoS2 nanosheets onto CuS, for the piezocatalytic degradation of Rhodamine B (RhB), methylene blue (MB) and hexavalent chromium (Cr (VI)). The excellent removal efficiency of Cr (VI) and RhB can be reached 100% within 180 s, through the piezocatalysis of CuS/MoS2-0.6 driven by mechanical stirring in the dark. Impressively, the piezoelectric current of CuS/MoS2-0.6 is 48 and 35.7 times higher than that of pure CuS and MoS2, respectively. The significantly enhanced piezocatalytic performance can be ascribed to the formation of CuS/MoS2 heterojunction and the piezoelectric field generated by MoS2 nanosheets, which promotes the efficient separation of electrons and holes. This study provides insights into strategies to improve catalytic performance through utilizing mechanical energy and opens a new horizon for environmental remediation.
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