Carbon Nitride for the Selective Oxidation of Aromatic Alcohols in Water under Visible Light

催化作用 化学 氮化碳 激进的 光化学 石墨氮化碳 可见光谱 光催化 酒精氧化 材料科学 碳纤维 有机化学 组合化学 计算机科学 算法 复合数 光电子学
作者
Baihua Long,Zhengxin Ding,Wei Wang
出处
期刊:Chemsuschem [Wiley]
卷期号:6 (11): 2074-2078 被引量:114
标识
DOI:10.1002/cssc.201300360
摘要

ChemSusChemVolume 6, Issue 11 p. 2074-2078 Communication Carbon Nitride for the Selective Oxidation of Aromatic Alcohols in Water under Visible Light Baihua Long, Baihua Long Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Search for more papers by this authorProf. Zhengxin Ding, Prof. Zhengxin Ding Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Search for more papers by this authorProf. Xinchen Wang, Corresponding Author Prof. Xinchen Wang [email protected] Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Search for more papers by this author Baihua Long, Baihua Long Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Search for more papers by this authorProf. Zhengxin Ding, Prof. Zhengxin Ding Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Search for more papers by this authorProf. Xinchen Wang, Corresponding Author Prof. Xinchen Wang [email protected] Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Research Institute of Photocatalysis, College of Chemistry and Chemical Engineering, Fuzhou University, Fuzhou, 350002 (PR China), Fax: (+86) 59183778608Search for more papers by this author First published: 26 August 2013 https://doi.org/10.1002/cssc.201300360Citations: 101Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Share a linkShare onEmailFacebookTwitterLinkedInRedditWechat Graphical Abstract The selective oxidation of aromatic alcohols in water is achieved by using a carbon nitride (CN) catalyst, dioxygen, and visible light. The unique electronic structure of CN avoids the direct formation of hydroxyl radicals, which typically cause the total oxidation of organics. The chemical stability of CN allows several chemical protocols for photoredox catalysis in water, as exemplified by cooperative catalysis involving Brønsted acids. This leads to a new, green pathway for diverse organic transformations using sunlight and water. Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Filename Description cssc_201300360_sm_miscellaneous_information.pdf2.3 MB miscellaneous_information Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. References 1 1aG.-J. T. Brink, I. W. C. E. Arends, R. A. Sheldon, Science 2000, 287, 1636–1639; 1bR. A. Sheldon, I. W. C. E. Arends, G.-J. T. Brink, A. Dijksman, Acc. Chem. Res. 2002, 35, 774–781; 1cT. Mallat, A. Baiker, Chem. Rev. 2004, 104, 3037–3058; 1dB. N. Zope, D. D. Hibbitts, M. Neurock, R. J. Davis, Science 2010, 330, 74–78. 2 2aG. Cardillo, Chromium Oxidations in Organic Chemistry, Vol. 19, Springer, Berlin, 1984; 2bS. Velusamy, T. Punniyamurthy, Org. Lett. 2004, 6, 217–219; 2cS. Patel, B. K. Mishra, J. Org. Chem. 2006, 71, 6759–6766. 3 3aF. Porta, L. Prati, J. Catal. 2004, 224, 397–403; 3bD. Wang, A. Villa, F. Porta, D. Su, L. Prati, Chem. Commun. 2006, 1956–1958; 3cA. Villa, D. Wang, D. S. Su, L. Prati, ChemCatChem 2009, 1, 510–514; 3dA. Villa, D. Wang, G. M. Veith, L. Prati, J. Catal. 2012, 292, 73–80. 4A. Villa, G. M. Veith, L. Prati, Angew. Chem. 2010, 122, 4601–4604; Angew. Chem. Int. Ed. 2010, 49, 4499–4502. 5 5aG. Ciamician, Science 1912, 36, 385–394; 5bO. Morton, Nature 2006, 443, 19–22; 5cK. Maeda, K. Teramura, D. Lu, T. Takata, N. Saito, Y. Inoue, K. Domen, Nature 2006, 440, 295–295; 5dM. Zhang, C. C. Chen, W. H. Ma, J. C. Zhao, Angew. Chem. 2008, 120, 9876–9879; Angew. Chem. Int. Ed. 2008, 47, 9730–9733; 5eJ. M. R. Narayanam, C. R. J. Stephenson, Chem. Soc. Rev. 2011, 40, 102–113. 6A. Fujishima, K. Honda, Nature 1972, 238, 37–38. 7 7aX. B. Chen, S. H. Shen, L. J. Guo, S. S. Mao, Chem. Rev. 2010, 110, 6503–6570; 7bD. Y. C. Leung, X. L. Fu, C. F. Wang, M. Ni, M. K. H. Leung, X. X. Wang, X. Z. Fu, ChemSusChem 2010, 3, 681–694; 7cG. M. Wang, H. Y. Wang, Y. C. Ling, Y. C. Tang, X. Y. Yang, R. C. Fitzmorris, C. C. Wang, J. Z. Zhang, Y. Li, Nano Lett. 2011, 11, 3026–3033; 7dS. Hoang, S. P. Berglund, N. T. Hahn, A. J. Bard, C. B. Mullins, J. Am. Chem. Soc. 2012, 134, 3659–3662. 8 8aA. J. Morris, G. J. Meyer, E. Fujita, Acc. Chem. Res. 2009, 42, 1983–1994; 8bN. M. Dimitrijevic, B. K. Vijayan, O. G. Poluektov, T. Rajh, K. A. Gray, H. He, P. Zapol, J. Am. Chem. Soc. 2011, 133, 3964–3971; 8cW.-N. Wang, W.-J. An, B. Ramalingam, S. Mukherjee, D. M. Niedzwiedzki, S. Gangopadhyay, P. Biswas, J. Am. Chem. Soc. 2012, 134, 11276–11281; 8dK. Teramura, S. Iguchi, Y. Mizuno, T. Shishido, T. Tanaka, Angew. Chem. 2012, 124, 8132–8135; Angew. Chem. Int. Ed. 2012, 51, 8008–8011. 9 9aQ. Wang, M. Zhang, C. C. Chen, W. H. Ma, J. C. Zhao, Angew. Chem. 2010, 122, 8148–8151; Angew. Chem. Int. Ed. 2010, 49, 7976–7979; 9bX. J. Lang, H. W. Ji, C. C. Chen, W. H. Ma, J. C. Zhao, Angew. Chem. 2011, 123, 4020–4023; Angew. Chem. Int. Ed. 2011, 50, 3934–3937; 9cD. Tsukamoto, Y. Shiraishi, Y. Sugano, S. Ichikawa, S. Tanaka, T. Hirai, J. Am. Chem. Soc. 2012, 134, 6309–6315. 10 10aG. Palmisano, S. Yurdakal, V. Augugliaro, V. Loddo, L. Palmisano, Adv. Synth. Catal. 2007, 349, 964–970; 10bS. Yurdakal, G. Palmisano, V. Loddo, V. Augugliaro, L. Palmisano, J. Am. Chem. Soc. 2008, 130, 1568–1569; 10cD. Tsukamoto, M. Ikeda, Y. Shiraishi, T. Hara, N. Ichikuni, S. Tanaka, T. Hirai, Chem. Eur. J. 2011, 17, 9816–9824; 10dL. Palmisano, V. Augugliaro, M. Bellardita, A. Di Paola, E. García López, V. Loddo, G. Marcì, G. Palmisano, S. Yurdakal, ChemSusChem 2011, 4, 1431–1438. 11 11aS. Furukawa, T. Shishido, K. Teramura, T. Tanaka, ACS Catal. 2012, 2, 175–179; 11bS. Furukawa, A. Tamura, T. Shishido, K. Teramura, T. Tanaka, Appl. Catal. B 2011, 110, 216–220. 12 12aK. Maeda, T. Takata, M. Hara, N. Saito, Y. Inoue, H. Kobayashi, K. Domen, J. Am. Chem. Soc. 2005, 127, 8286–8287; 12bF. Tessier, P. Maillard, Y. Lee, C. L. Bleugat, K. Domen, J. Phys. Chem. C 2009, 113, 8526–8531; 12cF. X. Zhang, K. Maeda, T. Takata, K. Domen, Chem. Commun. 2010, 46, 7313–7315. 13 13aX. C. Wang, K. Maeda, A. Thomas, K. Takanabe, G. Xin, J. M. Carlsson, K. Domen, M. Antonietti, Nat. Mater. 2009, 8, 76–80; 13bY. J. Zhang, A. Thomas, M. Antonietti, X. C. Wang, J. Am. Chem. Soc. 2009, 131, 50–51. 14 14aF. Z. Su, S. C. Mathew, L. Moehlmann, M. Antonietti, X. C. Wang, S. Blechert, Angew. Chem. 2011, 123, 683–686; Angew. Chem. Int. Ed. 2011, 50, 657–660; 14bZ. Ding, X. F. Chen, M. Antonietti, X. C. Wang, ChemSusChem 2011, 4, 274–281. 15M. B. Ansari, H. Jin, S.-E. Park, Catal. Sci. Technol. 2013, 3, 1261–1266. 16F. Z. Su, S. C. Mathew, G. Lipner, X. Z. Fu, M. Antonietti, S. Blechert, X. C. Wang, J. Am. Chem. Soc. 2010, 132, 16299–16301. 17L. Kesavan, R. Tiruvalam, M. H. A. Rahim, M. I. bin Saiman, D. I. Enache, R. L. Jenkins, N. Dimitratos, J. A. Lopez-Sanchez, S. H. Taylor, D. W. Knight, C. J. Kiely, G. J. Hutchings, Science 2011, 331, 195–199. 18D. I. Enache, J. K. Edwards, P. Landon, B. Solsona-Espriu, A. F. Carley, A. A. Herzing, M. Watanabe, C. J. Kiely, D. W. Knight, G. J. Hutchings, Science 2006, 311, 362–365. 19 19aA. S. Guram, X. Bei, H. W. Turner, Org. Lett. 2003, 5, 2485–2487; 19bJ. A. Mueller, C. P. Goller, M. S. Sigman, J. Am. Chem. Soc. 2004, 126, 9724–9734. Citing Literature Volume6, Issue11November 2013Pages 2074-2078 ReferencesRelatedInformation
最长约 10秒,即可获得该文献文件

科研通智能强力驱动
Strongly Powered by AbleSci AI
更新
PDF的下载单位、IP信息已删除 (2025-6-4)

科研通是完全免费的文献互助平台,具备全网最快的应助速度,最高的求助完成率。 对每一个文献求助,科研通都将尽心尽力,给求助人一个满意的交代。
实时播报
欧阳振应助元谷雪采纳,获得10
1秒前
嘿嘿啊哈发布了新的文献求助10
1秒前
奋斗向南发布了新的文献求助10
1秒前
科研通AI5应助xxxllllll采纳,获得10
1秒前
2秒前
CodeCraft应助我想@科研采纳,获得10
2秒前
科研通AI5应助我想@科研采纳,获得10
2秒前
2秒前
2秒前
cuicuisha完成签到,获得积分10
3秒前
救赎完成签到 ,获得积分10
3秒前
3秒前
3秒前
要好好看文献完成签到,获得积分10
3秒前
3秒前
wangwangdui发布了新的文献求助10
4秒前
替我活着发布了新的文献求助10
4秒前
4秒前
yyhgyg发布了新的文献求助10
5秒前
5秒前
5秒前
6秒前
曼凡发布了新的文献求助10
6秒前
怡然夏槐完成签到,获得积分10
6秒前
ao完成签到,获得积分10
6秒前
6秒前
orixero应助大湖小舟采纳,获得10
7秒前
yyq完成签到,获得积分10
7秒前
杜阳辉发布了新的文献求助10
7秒前
cch完成签到,获得积分20
7秒前
茶烟梧月发布了新的文献求助10
8秒前
小马甲应助桔梗采纳,获得10
8秒前
小二郎应助拼搏听寒采纳,获得10
8秒前
xiao yan发布了新的文献求助10
8秒前
小强发布了新的文献求助10
8秒前
8秒前
8秒前
HANK2024发布了新的文献求助10
9秒前
jerry发布了新的文献求助10
10秒前
今后应助FFFFcom采纳,获得10
10秒前
高分求助中
A new approach to the extrapolation of accelerated life test data 1000
ACSM’s Guidelines for Exercise Testing and Prescription, 12th edition 500
Picture Books with Same-sex Parented Families: Unintentional Censorship 500
Nucleophilic substitution in azasydnone-modified dinitroanisoles 500
不知道标题是什么 500
A Preliminary Study on Correlation Between Independent Components of Facial Thermal Images and Subjective Assessment of Chronic Stress 500
Phylogenetic study of the order Polydesmida (Myriapoda: Diplopoda) 360
热门求助领域 (近24小时)
化学 材料科学 医学 生物 工程类 有机化学 生物化学 物理 内科学 纳米技术 计算机科学 化学工程 复合材料 遗传学 基因 物理化学 催化作用 冶金 细胞生物学 免疫学
热门帖子
关注 科研通微信公众号,转发送积分 3971277
求助须知:如何正确求助?哪些是违规求助? 3515939
关于积分的说明 11180280
捐赠科研通 3251061
什么是DOI,文献DOI怎么找? 1795664
邀请新用户注册赠送积分活动 875937
科研通“疑难数据库(出版商)”最低求助积分说明 805209