Impacts of the East Asian summer monsoon on interannual variations of summertime surface-layer ozone concentrations over China

气候学 环境科学 高原(数学) 中国 大气科学 季风 化学输运模型 季节性 地理 对流层 地质学 数学 统计 数学分析 考古
作者
Yuanjian Yang,Hong Liao,J. Li
出处
期刊:Atmospheric Chemistry and Physics 卷期号:14 (13): 6867-6879 被引量:90
标识
DOI:10.5194/acp-14-6867-2014
摘要

Abstract. We apply a global three-dimensional Goddard Earth Observing System (GEOS) chemical transport model (GEOS-Chem) driven by the NASA/GEOS-4 assimilated meteorological fields to quantify the impacts of the East Asian summer monsoon (EASM) on interannual variations of June-July-August (JJA) surface-layer O3 concentrations over China. With anthropogenic emissions fixed at year 2005 levels, the model simulation for years 1986–2006 shows that the changes in meteorological parameters alone lead to interannual variations in JJA surface-layer O3 concentrations by 2–5% over central eastern China, 1–3% in northwestern China, and 5–10% over the Tibetan Plateau as well as the border and coastal areas of southern China, as the interannual variations are relative to the average O3 concentrations over the 21 yr period. Over the years 1986–2006, the O3 concentration averaged over all of China is found to correlate positively with the EASM index with a large correlation coefficient of +0.75, indicating that JJA O3 concentrations are lower (or higher) in weaker (or stronger) EASM years. Relative to JJA surface-layer O3 concentrations in the strongest EASM years (1990, 1994, 1997, 2002, and 2006), O3 levels in the weakest EASM years (1988, 1989, 1996, 1998, and 2003) are lower over almost all of China with a national mean lower O3 concentration by 2.0 ppbv (parts per billion by volume; or 4%). Regionally, the largest percentage differences in O3 concentration between the weakest and strongest EASM years are found to exceed 6% in northeastern China, southwestern China, and over the Tibetan Plateau. Sensitivity studies show that the difference in transboundary transport of O3 is the most dominant factor that leads to lower-O3 concentrations in the weakest EASM years than in the strongest EASM years, which, together with the enhanced vertical convections in the weakest EASM years, explain about 80% of the differences in surface-layer O3 concentrations between the weakest and strongest EASM years. We also find that the impacts the EASM strength on JJA surface-layer O3 can be particularly strong (comparable in magnitude to the impacts on O3 by changes in anthropogenic emissions over years 1986–2006) for certain years. The largest increases in O3 by anthropogenic emissions are simulated over southeastern China, whereas the largest impacts of the EASM on O3 are found over central and western China.
最长约 10秒,即可获得该文献文件

科研通智能强力驱动
Strongly Powered by AbleSci AI
更新
大幅提高文件上传限制,最高150M (2024-4-1)

科研通是完全免费的文献互助平台,具备全网最快的应助速度,最高的求助完成率。 对每一个文献求助,科研通都将尽心尽力,给求助人一个满意的交代。
实时播报
hihi发布了新的文献求助10
2秒前
忧伤的寒梦完成签到,获得积分10
2秒前
泠风来完成签到,获得积分10
2秒前
半夏完成签到,获得积分10
3秒前
海绵宝宝完成签到,获得积分10
5秒前
哭泣的幻翠完成签到 ,获得积分10
6秒前
yue957完成签到 ,获得积分20
6秒前
脑洞疼应助hpp采纳,获得10
7秒前
Jim发布了新的文献求助30
8秒前
淡淡的士晋完成签到,获得积分10
8秒前
毛通完成签到,获得积分10
9秒前
所所应助kyt0001采纳,获得10
11秒前
科研通AI2S应助kyt0001采纳,获得10
11秒前
hzc应助kyt0001采纳,获得10
11秒前
大个应助fengliurencai采纳,获得10
12秒前
CodeCraft应助詹上上采纳,获得10
12秒前
14秒前
15秒前
口口完成签到 ,获得积分10
21秒前
ssk发布了新的文献求助10
21秒前
xuhongbo发布了新的文献求助10
22秒前
lzy发布了新的文献求助200
23秒前
23秒前
24秒前
诚心绿兰完成签到 ,获得积分10
24秒前
25秒前
流露发布了新的文献求助10
29秒前
许熙完成签到,获得积分10
29秒前
ZHANG完成签到,获得积分10
30秒前
你好完成签到 ,获得积分10
30秒前
留胡子的胡完成签到,获得积分10
31秒前
31秒前
31秒前
我爱Chem完成签到 ,获得积分10
34秒前
丈八二桃完成签到,获得积分10
34秒前
小二郎应助科研通管家采纳,获得10
35秒前
詹上上发布了新的文献求助10
35秒前
烟花应助科研通管家采纳,获得10
35秒前
科研通AI2S应助科研通管家采纳,获得30
35秒前
毛豆爸爸应助科研通管家采纳,获得10
35秒前
高分求助中
Sustainability in ’Tides Chemistry 2000
Studien zur Ideengeschichte der Gesetzgebung 1000
TM 5-855-1(Fundamentals of protective design for conventional weapons) 1000
Threaded Harmony: A Sustainable Approach to Fashion 810
Handbook of the Mammals of the World – Volume 3: Primates 805
Ethnicities: Media, Health, and Coping 800
Gerard de Lairesse : an artist between stage and studio 500
热门求助领域 (近24小时)
化学 医学 生物 材料科学 工程类 有机化学 生物化学 物理 内科学 纳米技术 计算机科学 化学工程 复合材料 基因 遗传学 催化作用 物理化学 免疫学 量子力学 细胞生物学
热门帖子
关注 科研通微信公众号,转发送积分 3074227
求助须知:如何正确求助?哪些是违规求助? 2727639
关于积分的说明 7499897
捐赠科研通 2375736
什么是DOI,文献DOI怎么找? 1259523
科研通“疑难数据库(出版商)”最低求助积分说明 610724
版权声明 597081