有机太阳能电池
聚合物
材料科学
三元运算
共轭体系
串联
接受者
富勒烯
纳米技术
有机化学
化学
计算机科学
凝聚态物理
物理
复合材料
程序设计语言
作者
Zhong Zheng,Huifeng Yao,Long Ye,Ye Xu,Shaoqing Zhang,Jianhui Hou
标识
DOI:10.1016/j.mattod.2019.10.023
摘要
Due to the advantages such as being low cost, light weight, and flexible as well as having low toxicity, organic solar cells (OSCs) have attracted extensive interest. The field of OSCs progressed dramatically after the emergence of non-fullerene small molecule acceptors. In addition to the development of these acceptor materials, a key driver in the rapid progress of OSC research was the introduction of the PBDB-T polymer and its derivatives. In this review, we first give a brief overview of the structural features of PBDB-T congeners and the strategies used to design these polymers. The interesting aggregation effects of PBDB-T congeners in solution and solid-states are highlighted. Recent advances in the morphological understanding OSCs based on PBDB-T congeners are discussed using selected examples. In addition, the versatile applications of PBDB-T congeners in OSC devices, including interfacially modified binary, ternary and tandem devices, are also summarized. Importantly, we assess the energy loss and provide a meta-analysis of a library of high-performance PBDB-T type polymers, which are compared with other types of conjugated polymers. Finally, the remaining questions and the prospects of these exciting polymers are suggested.
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