气凝胶
基质(水族馆)
成核
播种
催化作用
化学工程
复合数
析氧
微型反应器
材料科学
化学
电化学
环加成
纳米技术
电极
有机化学
复合材料
物理化学
航空航天工程
工程类
地质学
海洋学
作者
Xiao‐Jue Bai,Xingyu Lu,Ran Ju,Huan Chen,Lei Shao,Xu Zhai,Yunong Li,Fuqiang Fan,Yu Fu,Wei Qi
标识
DOI:10.1002/anie.202012354
摘要
Abstract Substrate‐supported metal–organic frameworks (MOFs) films are desired to realize their potential in practical applications. Herein, a novel substrate‐seeding secondary‐growth strategy is developed to prepare composites of uniform MOFs films on aerogel walls. Briefly, the organic ligand is “pre‐seeded” onto the aerogel walls, and then a small amount of metal‐ion solution is sprayed onto the prepared aerogel. The sprayed solution diffuses along the aerogel walls to form a continuous thin layer, which confines the nucleation reaction, promoting the formation of uniform MOFs films on the aerogel walls. The whole process is simple in operation, highly efficient, and eco‐friendly. The resulting hierarchical MOFs/aerogel composites have abundant accessible active sites and enable excellent mass transfer, which endows the composite with outstanding catalytic activity and stability in both liquid‐phase CO 2 cycloaddition and electrochemical oxygen evolution reaction (OER) process.
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