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A Flexible Sulfur‐Graphene‐Polypropylene Separator Integrated Electrode for Advanced Li–S Batteries

石墨烯 材料科学 硫黄 电极 分离器(采油) 导电体 多硫化物 电池(电) 聚丙烯 纳米技术 复合材料 计算机科学 冶金 化学 功率(物理) 物理化学 物理 热力学 量子力学 电解质
作者
Guangmin Zhou,Lu Li,Dawei Wang,Xuyi Shan,Songfeng Pei,Feng Li,Hui‐Ming Cheng
出处
期刊:Advanced Materials [Wiley]
卷期号:27 (4): 641-647 被引量:562
标识
DOI:10.1002/adma.201404210
摘要

Advanced MaterialsVolume 27, Issue 4 p. 641-647 Communication A Flexible Sulfur-Graphene-Polypropylene Separator Integrated Electrode for Advanced Li–S Batteries Guangmin Zhou, Guangmin Zhou Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorLu Li, Lu Li Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorDa-Wei Wang, Da-Wei Wang School of Chemical Engineering, UNSW Australia, UNSW Sydney, NSW, 2052 AustraliaSearch for more papers by this authorXu-yi Shan, Xu-yi Shan Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorSongfeng Pei, Songfeng Pei Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorFeng Li, Corresponding Author Feng Li Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaE-mail: [email protected], [email protected]Search for more papers by this authorHui-Ming Cheng, Corresponding Author Hui-Ming Cheng Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaE-mail: [email protected], [email protected]Search for more papers by this author Guangmin Zhou, Guangmin Zhou Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorLu Li, Lu Li Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorDa-Wei Wang, Da-Wei Wang School of Chemical Engineering, UNSW Australia, UNSW Sydney, NSW, 2052 AustraliaSearch for more papers by this authorXu-yi Shan, Xu-yi Shan Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorSongfeng Pei, Songfeng Pei Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaSearch for more papers by this authorFeng Li, Corresponding Author Feng Li Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaE-mail: [email protected], [email protected]Search for more papers by this authorHui-Ming Cheng, Corresponding Author Hui-Ming Cheng Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, 72 Wenhua Road, Shenyang, 110016 P.R. ChinaE-mail: [email protected], [email protected]Search for more papers by this author First published: 06 November 2014 https://doi.org/10.1002/adma.201404210Citations: 505Read the full textAboutPDF ToolsRequest permissionExport citationAdd to favoritesTrack citation ShareShare Give accessShare full text accessShare full-text accessPlease review our Terms and Conditions of Use and check box below to share full-text version of article.I have read and accept the Wiley Online Library Terms and Conditions of UseShareable LinkUse the link below to share a full-text version of this article with your friends and colleagues. Learn more.Copy URL Graphical Abstract A flexible Li–S battery based on an integrated structure of sulfur and graphene on a separator is developed. The internal graphene current collector offers a continuous conductive pathway, a modified interface with sulfur, and a good barrier to and an effective reservoir for dissolved polysulfides, consequently improving the capacity and cyclic life of the Li–S battery. References 1Y. H. Kwon, S. W. Woo, H. R. Jung, H. K. Yu, K. Kim, B. H. Oh, S. Ahn, S. Y. Lee, S. W. Song, J. Cho, H. C. Shin, J. Y. Kim, Adv. Mater. 2012, 24, 5192. 2H. Gwon, J. Hong, H. Kim, D.-H. Seo, S. Jeon, K. Kang, Energy Environ. Sci. 2014, 7, 538. 3S.-Y. Lee, K.-H. Choi, W.-S. Choi, Y. H. Kwon, H.-R. Jung, H.-C. Shin, J. Y. Kim, Energy Environ. Sci. 2013, 6, 2414. 4G. Zhou, F. Li, H.-M. Cheng, Energy Environ. Sci. 2014, 7, 1307. 5J. M. Tarascon, M. Armand, Nature 2001, 414, 359. 6P. G. Bruce, B. Scrosati, J. M. Tarascon, Angew. Chem Int. Ed. 2008, 47, 2930. 7P. G. Bruce, S. A. Freunberger, L. J. Hardwick, J.-M. Tarascon, Nat. Mater. 2012, 11, 19. 8H. Nishide, K. Oyaizu, Science 2008, 319, 737. 9Q. Xiao, Q. Zhang, Y. Fan, X. Wang, R. A. Susantyoko, Energy Environ. Sci. 2014, 7, 2261. 10L. B. Hu, H. Wu, F. La Mantia, Y. A. Yang, Y. Cui, ACS Nano 2010, 4, 5843. 11S. Liu, Z. Wang, C. Yu, H. B. Wu, G. Wang, Q. Dong, J. Qiu, A. Eychmüller, X. W. Lou, Adv. Mater. 2013, 25, 3462. 12G. M. Zhou, S. Pei, L. Li, D.-W. Wang, S. Wang, K. Huang, L.-C. Yin, F. Li, H.-M. Cheng, Adv. Mater. 2014, 26, 625. 13J.-Q. Huang, H.-J. Peng, X.-Y. Liu, J.-Q. Nie, X.-B. Cheng, Q. Zhang, F. Wei, J. Mater. Chem. A 2014, 2, 10869. 14R. V. Noorden, Nature 2014, 507, 26. 15C. X. Zu, H. Li, Energy Environ. Sci. 2011, 4, 2614. 16X. P. Gao, H. X. Yang, Energy Environ. Sci. 2010, 3, 174. 17D.-W. Wang, G. M. Zhou, F. Li, K.-H. Wu, G. M. Lu, H.-M. Cheng, I. Gentle, Phys. Chem. Chem. Phys. 2012, 14, 8703. 18X. L. Ji, K. T. Lee, L. F. Nazar, Nat. Mater. 2009, 8, 500. 19D.-W. Wang, Q. Zeng, G. M. Zhou, L. Yin, F. Li, H.-M. Cheng, I. R. Gentle, G. Q. M. Lu, J. Mater. Chem. A 2013, 1, 9382. 20Y. Yang, G. Zheng, Y. Cui, Chem. Soc. Rev. 2013, 42, 3018. 21A. Manthiram, Y. Fu, S.-H. Chung, C. Zu, Y.-S. Su, Chem. Rev. 2014, DOI: 10.1021/cr500062v. 22S. Evers, L. F. Nazar, Acc. Chem. Res. 2013, 46, 1135. 23A. Manthiram, Y. Fu, Y.-S. Su, Acc. Chem. Res. 2012, 46, 1125. 24S. Chen, X. Huang, H. Liu, B. Sun, W. Yeoh, K. Li, J. Zhang, G. Wang, Adv. Energy Mater. 2014, 4, 1301761. 25Z. Seh, W. Li, J. J. Cha, G. Zheng, Y. Yang, M. T. McDowell, P.-C. Hsu, Y. Cui, Nat. Commun. 2013, 4, 1331. 26C. Huang, J. Xiao, Y. Y. Shao, J. M. Zheng, W. D. Bennett, D. P. Lu, S. V. Laxmikant, M. Engelhard, L. W. Ji, J. Zhang, X. L. Li, G. L. Graff, J. Liu, Nat. Commun. 2014, 5, 3015. 27X. Zhang, W. Wang, A. Wang, Y. Huang, K. Yuan, Z. Yu, J. Qiu, Y. Yang, J. Mater. Chem. A 2014, 2, 11660. 28X.-B. Cheng, H.-J. Peng, J.-Q. Huang, F. Wei, Q. Zhang, Small 2014, DOI: 10.1002/smll.201401837. 29J. Hassoun, B. Scrosati, Angew. Chem Int. Ed. 2010, 49, 2371. 30Y. Yang, M. T. McDowell, A. Jackson, J. J. Cha, S. S. Hong, Y. Cui, Nano Lett. 2010, 10, 1486. 31R. Elazari, G. Salitra, G. Gershinsky, A. Garsuch, A. Panchenko, D. Aurbach, Electrochem. Commun. 2012, 14, 21. 32R. Elazari, G. Salitra, A. Garsuch, A. Panchenko, D. Aurbach, Adv. Mater. 2011, 23, 5641. 33M. Hagen, S. Dörfler, P. Fanz, T. Berger, R. Speck, J. Tübke, H. Althues, M. J. Hoffmann, C. Scherr, S. Kaskel, J. Power Sources 2013, 224, 260. 34S. Thieme, J. Bruckner, I. Bauer, M. Oschatz, L. Borchardt, H. Althues, S. Kaskel, J. Mater. Chem. A 2013, 1, 9225. 35L. B. Hu, J. W. Choi, Y. Yang, S. Jeong, F. La Mantia, L. F. Cui, Y. Cui, Proc. Natl. Acad. Sci. USA 2009, 106, 21490. 36H.-C. Wu, H.-C. Wu, E. Lee, N.-L. Wu, Electrochem. Commun. 2010, 12, 488. 37G. M. Zhou, D.-W. Wang, F. Li, P.-X. Hou, L. Yin, C. Liu, G. Q. Lu, I. R. Gentle, H.-M. Cheng, Energy Environ. Sci. 2012, 5, 8901. 38X. L. Jia, Z. Chen, X. Cui, Y. T. Peng, X. L. Wang, G. Wang, F. Wei, Y. F. Lu, ACS Nano 2012, 6, 9911. 39K. Wang, S. Luo, Y. Wu, X. F. He, F. Zhao, J. P. Wang, K. L. Jiang, S. S. Fan, Adv. Funct. Mater. 2013, 23, 846. 40S. Luo, K. Wang, J. P. Wang, K. L. Jiang, Q. Q. Li, S. S. Fan, Adv. Mater. 2012, 24, 2294. 41M. V. Reddy, T. Yu, C. H. Sow, Z. X. Shen, C. T. Lim, G. V. S. Rao, B. V. R. Chowdari, Adv. Funct. Mater. 2007, 17, 2792. 42G. M. Zhou, D.-W. Wang, L.-C. Yin, N. Li, F. Li, H.-M. Cheng, ACS Nano 2012, 6, 3214. 43X. L. Ji, L. F. Nazar, J. Mater. Chem. 2010, 20, 9821. 44G. Y. Zheng, Y. Yang, J. J. Cha, S. S. Hong, Y. Cui, Nano Lett. 2011, 11, 4462. 45D. Aurbach, E. Pollak, R. Elazari, G. Salitra, C. S. Kelley, J. Affinito, J. Electrochem. Soc. 2009, 156, A694. Citing Literature Supporting Information As a service to our authors and readers, this journal provides supporting information supplied by the authors. Such materials are peer reviewed and may be re-organized for online delivery, but are not copy-edited or typeset. Technical support issues arising from supporting information (other than missing files) should be addressed to the authors. Filename Description adma201404210-sup-0001-S1.pdf758.2 KB Supplementary Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article. Volume27, Issue4January 27, 2015Pages 641-647 ReferencesRelatedInformation
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