电介质
材料科学
矿物学
陶瓷
微波食品加热
分析化学(期刊)
复合材料
化学
物理
光电子学
色谱法
量子力学
作者
Yu Lou,Wei Wang,Diming Xu,Chao Du,Xin Wang,Fayaz Hussain,Moustafa A. Darwish,Tao Zhou,Ya‐Wei Chen,Qi‐Xin Liang,Meirong Zhang,Yongqiang Pang,Di Zhou
摘要
Abstract In this work, the 0.5BaCuSi 4 O 10 –0.5BaCuSi 2 O 6 ‐based ceramics were synthesized using a standard solid‐phase reaction process, and the inherent relationship between crystal structure and microwave dielectric properties was thoroughly explored. The crystal structure of the 0.5BaCuSi 4 O 10 –0.5BaCuSi 2 O 6 ceramic was determined by X‐ray diffractometer, which confirmed the existence of two phases. Microstructure observation of the ceramics was obtained by scanning electron microscope (SEM). Excellent microwave dielectric properties with a low ԑ r ∼6.52, a high Q × f ∼46 010 GHz, and the temperature coefficient of resonant frequency (TCF) ∼−14 ppm°C −1 were obtained in the 0.5BaCuSi 4 O 10 –0.5BaCuSi 2 O 6 ceramic sintered at 1060°C. By adding sintering additives LiF and Li 2 O–B 2 O 3 –SiO 2 –CaO–Al 2 O 3 (LBSCA) glass, the sintering temperature was decreased from 1060°C to 870°C. Good microwave dielectric properties with a ԑ r ∼6.59, a Q × f ∼18 820 GHz, and TCF ∼−14 ppm°C −1 were achieved in the 0.5BaCuSi 4 O 10 –0.5BaCuSi 2 O 6 ‐2 wt.% LiF, 1 wt.% LBSCA (2F1LBSCA) ceramic sintered at 870°C. The low‐temperature firing ceramics could also be well co‐fired with Ag with good chemical compatibility. These results indicated that the 0.5BaCuSi 4 O 10 –0.5BaCuSi 2 O 6 ceramic with 2F1LBSCA additions can be utilized in low‐temperature co‐fired ceramics technology to produce high‐frequency communication components.
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