A poly(L-lactic Acid)-based flexible piezoelectric energy harvester with micro-zigzag structures

Abstract Piezoelectric energy harvester (PEH) holds great potential for flexible electronics and wearable devices. However, the power conversion efficiency of flexible PEH (fPEH) has often been a limiting factor, especially under variable excitation. Herein, we propose a practical solution: a poly(L-lactic acid)-based fPEH with 3D-printed micro-zigzag structures. This design not only broadens the operational bandwidth and enhances low-frequency response but also offers a tangible improvement in the power conversion efficiency of fPEH. The micro-zigzag structure was designed and fabricated using a digital light processing 3D printing technique with acrylates, a method that is readily accessible to researchers and engineers in the field. Mechanical properties of the 3D-printed acrylic elastomers with different compositions were investigated to obtain the material parameters, and then fPEH with the sandwich structure was fabricated via sputtering and packaging. Subsequently, numerical simulation was conducted on the micro-zigzag structures to determine the structure sizes and oscillation frequencies of fPEH. Finally, four micro-zigzag structures with 3-, 4-, 5- and 6-mm lengths were tested to obtain oscillation frequencies of 51, 37, 22, and 21 Hz consistent with the simulation. The output voltages of fPEH are 11 ~ 30 mV with the load ranges of 60 ~ 100 MΩ. Stability evaluation showed that the fPEH can work under low frequency (<100 Hz) and broadband conditions. The micro-zigzag structure provided new insights for the design of fPEH, paving the way for more efficient and practical energy harvesting solutions in the future.