余辉
发光
材料科学
光子上转换
激发
纳米颗粒
持续发光
兴奋剂
光电子学
激发态
纳米技术
原子物理学
热释光
物理
伽马射线暴
量子力学
天文
作者
Chao Zhou,Denghao Li,Lei Lei,Gongxun Bai,Huanping Wang,Xianghua Zhang,Shiqing Xu,Jianrong Qiu
标识
DOI:10.1016/j.ceramint.2023.07.040
摘要
Multimodal luminescence has emerged as a promising solution in the realm of anti-counterfeiting techniques, which have gained global attention due to their association with information and data security. The conventional approach to achieving multimodal luminescence typically involves combining upconversion and downshifting luminescence, which necessitates the use of external excitation sources and costly detection equipment. Herein, we develop an anti-counterfeiting strategy based on the afterglow performance of NaLuF4: Gd, Tm nanoparticles after X-ray excitation. The X-ray-induced Frenkel defects-base traps ensnare electrons with low kinetic energy, resulting in the creation of persistent photon traps that are responsible for the temperature-dependent afterglow intensity. The dual-band and thermo-enhanced afterglow emission can encrypt information well according to our proof-of-concept experiment and the visible light signal can be successfully captured by a smartphone camera. These unique features of NaLuF4: Gd, Tm nanoparticles render them highly appealing for multilevel anti-counterfeiting applications.
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