Plasma Engineering toward Improving the Microwave-Absorbing/Shielding Feature of a Biomass-Derived Material

电磁屏蔽 微波食品加热 生物量(生态学) 等离子体 材料科学 特征(语言学) 工艺工程 化学工程 光电子学 复合材料 工程类 物理 电信 核物理学 地质学 语言学 海洋学 哲学
作者
Elnaz Selseleh‐Zakerin,Ali Mirkhan,Mojtaba Shafiee,Mohammadreza Alihoseini,Mohammad Reza Khani,Babak Shokri,Seyed Hassan Tavassoli,Reza Peymanfar
出处
期刊:Langmuir [American Chemical Society]
卷期号:40 (23): 12148-12158 被引量:14
标识
DOI:10.1021/acs.langmuir.4c01046
摘要

During the past decade, ever-increasing electromagnetic pollution has excited a global concern. A sustainable resource, facile experimental scenario, fascinating reflection loss (RL), and broad efficient bandwidth are the substantial factors that intrigue researchers. This research led to the achievement of a brilliant microwave-absorbing material by treating pampas as biomass. The carbon-based microfibers attained by biowaste were treated by plasma under diverse environments to amplify their microwave-absorbing features. Moreover, a pyrolysis scenario was performed to compare the results. The reductive processes were performed by H2 plasma and carbonization. However, the CO2 plasma was performed to regulate the heteroatoms and defects. Interestingly, polystyrene (PS) was applied as a microwave-absorbing matrix. The aromatic rings existing in the absorbing medium establish electrostatic interactions, elevating interfacial polarization, and physical characteristics of PS augment the practical applications of the final product. The manipulated biomasses were characterized by Raman, X-ray diffraction, energy-dispersive spectroscopy, field emission scanning electron microscopy, and diffuse reflection spectroscopy analyses. Eventually, the microwave-absorbing features were estimated by a vector network analyzer. The plasma-treated pampas under H2/Ar blended with PS gained a maximum RL of −90.65 dB at 8.79 GHz and an efficient bandwidth (RL ≤ −10 dB) of 4.24 GHz with a thickness of 3.20 mm; meanwhile, plasma treatment under CO2 led to a maximum RL of 97.99 dB at 14.92 GHz and an efficient bandwidth of 7.74 GHz with a 2.05 mm thickness. Particularly, the biomass plasmolyzed under Ar covered the entire X and Ku bands with a thickness of 2.10 mm. Notably, total shielding efficiencies of the treated bioinspired materials were up to ≈99%, desirable for practical applications.
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