Magnetointeractive Cr2Te3‐Coated Liquid Metal Droplets for Flexible Memory Arrays and Wearable Sensors

Abstract Magnetic liquid metal droplets, featured by unique fluidity, metallic conductivity, and magnetic reactivity, are of growing significance for next‐generation flexible electronics. Conventional fabrication routes, which typically incorporate magnetic nanoparticles into liquid metals, otherwise encounter the pitfall pertaining to surface adhesivity and corrosivity over device modules. Here, an innovative approach of synergizing liquid metals with 2D magnetic materials is presented, accordingly creating chromium(III)‐telluride‐coated liquid metal (CT–LM) droplets via a simple self‐assembly process. The CT–LM droplets exhibit controllable deformation and locomotion under magnetic fields, demonstrate nonadherence to various surfaces, and enable cost‐effective recycling of components. The functionality of CT–LM droplets is validated through their use in magnetointeractive memory devices to enable sensing/storing 64 magnetic paths and in wearable sensors as the flexible vibrator for dynamic gesture recognition with machine learning assistance. This work opens new avenues for the functional droplet design and broadens the horizons of flexible electronics.