碳纳米管
DNA折纸
纳米技术
纳米电子学
材料科学
DNA
DNA纳米技术
纳米结构
化学
生物化学
作者
Yueyue Zhang,Xiuhai Mao,Fan Li,Min Li,Xinxin Jing,Zhilei Ge,Lihua Wang,Kai Liu,Hongjie Zhang,Chunhai Fan,Xiaolei Zuo
标识
DOI:10.1002/anie.201916043
摘要
Abstract Aligning carbon nanotubes (CNTs) is a key challenge for fabricating CNT‐based electronic devices. Herein, we report a spherical nucleic acid (SNA) mediated approach for the highly precise alignment of CNTs at prescribed sites on DNA origami. We find that the cooperative DNA hybridization occurring at the interface of SNA and DNA‐coated CNTs leads to an approximately five‐fold improvement of the positioning efficiency. By combining this with the intrinsic positioning addressability of DNA origami, CNTs can be aligned in parallel with an extremely small angular variation of within 10°. Moreover, we demonstrate that the parallel alignment of CNTs prevents incorrect logic functionality originating from stray conducting paths formed by misaligned CNTs. This SNA‐mediated method thus holds great potential for fabricating scalable CNT arrays for nanoelectronics.
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