Circular dichroism metamirrors with near-perfect extinction

圆极化 圆二色性 物理 磁圆二色性 光学 振动圆二色性 线性二色性 极化(电化学) 二色性 超材料 X射线磁圆二色性 量子力学 化学 结晶学 微带线 物理化学 谱线
作者
Zuojia Wang,Hui Jia,Kan Yao,Wenshan Cai,Hongsheng Chen,Yongmin Liu
标识
DOI:10.1109/piers.2016.7735089
摘要

The efficient analysis and engineering of the polarization state is imperative in diverse disciplines, including physics, materials science, biology and quantum optics. For instance, scientists apply circularly polarized light to manipulate the spin state of electron for quantum information processing. Chrysina gloriosa (jeweled beetles) under left-handed circularly polarized light illumination appear more brilliant than those under right-handed circularly polarized light illumination, and circular dichroism spectroscopy is of critical importance to identify the structure of chiral molecules. Metallic mirrors are basic elements and widely used in optical setup to control the path of light. However, the state of circular polarization is reversed, or even degrades to elliptical polarization when it is reflected off a surface. Therefore, the original handedness of the optical signals is lost after multiple reflections in a complex optical system. Here, we propose and demonstrate a new concept of circular dichroism metamirrors, which enables selective, near-perfect reflection of designated circularly polarized light without reversing its handedness, yet complete absorption of the other polarization state. Such a metamirror can be considered as the optical analogy of Chrysina gloriosa in nature, while exhibits nearly maximal efficiency. A general method to design the circular dichroism metasmirror is presented under the framework of Jones calculus. It is analytically shown that the building block of such a metamirror needs to simultaneously break the n-fold rotational (n > 2) symmetry and mirror symmetry. By combining two layers of anisotropic metamaterial structures, we design a circular dichroism metamirror in the mid-infrared region, which shows perfect reflectance (94.7%) for left-handed circularly polarized light without reversing its handedness, while almost completely absorbs (99.3%) right-handed circularly polarized light. These findings offer new methodology to implement novel photonic devices for a variety of applications, including polarimetric imaging, molecular spectroscopy and quantum information processing.
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