Interface evolution and pinch-off mechanism of droplet in two-phase liquid flow through T-junction microfluidic system

微流控 曲率 曲率半径 半径 机械 分手 流量(数学) 材料科学 相(物质) 物理 纳米技术 平均曲率 计算机科学 几何学 流量平均曲率 数学 计算机安全 量子力学 核物理学
作者
Akepogu Venkateshwarlu,Ram Prakash Bharti
出处
期刊:Colloids and Surfaces A: Physicochemical and Engineering Aspects [Elsevier]
卷期号:642: 128536-128536 被引量:11
标识
DOI:10.1016/j.colsurfa.2022.128536
摘要

This work has explored interface evolution and pinch-off mechanism of the droplet formation in two-phase flow through cross-flow microfluidic device. The two-dimensional mathematical model equations have been solved using the finite element method under the squeezing regime (Cac< 10−2) for wide range of flow rates (0.1 ≤ Qr ≤ 10) and fixed contact angle (θ = 135°). The droplet formation process has been classified into various instantaneous stages as initial, filling, squeezing, pinch-off and stable droplet through microscopic visualization of interface evolution in phase profiles. The dynamics of interface, and point pressure in both phases is further gained and discussed. Maximum pressure in the continuous phase varied linearly with Qr. The droplet pinch-off mechanism has been thoroughly elucidated by determining the local radius of the curvature (Rc,min) and neck width (2r) during the squeezing and pinch-off stages. At the pinch-off point, both Rc,min and 2r are non-linearly related to Qr. Further, the topological dynamics of interface has been explored by analyzing the Laplace pressure (pL), acting on the interface curvature, evaluated using (a) pressure sensors in both phases, pL = pdp − pcp, (b) local radius of curvature pL=σ1∕Rf+1∕Rr, and (c) minimum radius of curvature, pL=σ1∕Rc,min. The insights obtained from the present work can reliably be used in designing the model and prototypes of microfluidic devices for generating monodispersed droplets in emulsions, and the droplet breakup mechanism would help accurate prediction of the pinch-off moment. The proposed knowledge provides detailed insights of the interface evolution and droplet pinch-off to a precision of 10 μs and resolution of 10 μm, equivalent to experimental flow visualization with a high-speed (105 fps) and high-resolution (10 μm pixel size) camera.

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