Double Superconducting Dome and Triple Enhancement of Tc in the Kagome Superconductor CsV3Sb

计算机科学
作者
Keyu Chen,Ningning Wang,Q. W. Yin,Yuqian Gu,Kai Jiang,Z. J. Tu,Chunsheng Gong,Yoshiya Uwatoko,Jianping Sun,Hechang Lei,Jiangping Hu,Jinguang Cheng
出处
期刊:Physical Review Letters [American Physical Society]
卷期号:126 (24) 被引量:333
标识
DOI:10.1103/physrevlett.126.247001
摘要

${\mathrm{CsV}}_{3}{\mathrm{Sb}}_{5}$ is a newly discovered ${Z}_{2}$ topological kagome metal showing the coexistence of a charge-density-wave (CDW)-like order at ${T}^{*}=94\text{ }\text{ }\mathrm{K}$ and superconductivity (SC) at ${T}_{c}=2.5\text{ }\text{ }\mathrm{K}$ at ambient pressure. Here, we study the interplay between CDW and SC in ${\mathrm{CsV}}_{3}{\mathrm{Sb}}_{5}$ via measurements of resistivity, dc and ac magnetic susceptibility under various pressures up to 6.6 GPa. We find that the CDW transition decreases with pressure and experience a subtle modification at ${P}_{c1}\ensuremath{\approx}0.6--0.9\text{ }\text{ }\mathrm{GPa}$ before it vanishes completely at ${P}_{c2}\ensuremath{\approx}2\text{ }\text{ }\mathrm{GPa}$. Correspondingly, ${T}_{c}(P)$ displays an unusual $M$-shaped double dome with two maxima around ${P}_{c1}$ and ${P}_{c2}$, respectively, leading to a tripled enhancement of ${T}_{c}$ to about 8 K at 2 GPa. The obtained temperature-pressure phase diagram resembles those of unconventional superconductors, illustrating an intimated competition between CDW-like order and SC. The competition is found to be particularly strong for the intermediate pressure range ${P}_{c1}\ensuremath{\le}P\ensuremath{\le}{P}_{c2}$ as evidenced by the broad superconducting transition and reduced superconducting volume fraction. The modification of CDW order around ${P}_{c1}$ has been discussed based on the band structure calculations. This work not only demonstrates the potential to raise ${T}_{c}$ of the V-based kagome superconductors, but also offers more insights into the rich physics related to the electron correlations in this novel family of topological kagome metals.

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