CMAQ
环境科学
数据同化
反演(地质)
生物圈
生物圈模型
碳通量
大气科学
水槽(地理)
碳汇
焊剂(冶金)
气象学
化学输运模型
气候学
臭氧
气候变化
地质学
生态系统
对流层
化学
物理
地图学
海洋学
古生物学
构造盆地
有机化学
地理
生态学
生物
天文
作者
Zhen Peng,Xingxia Kou,M. Zhang,Lili Lei,Shiguang Miao,Hengmao Wang,Fei Jiang,Han Xiao,Shuangxi Fang
摘要
Abstract Most of China's carbon sink inversion research uses global atmospheric transport models to assimilate natural fluxes, which quantifies the biosphere and ocean carbon budget with a relative coarse spatial resolution and long timescale from a weekly or monthly perspective. Toward high‐resolution inversion of CO 2 fluxes, a novel carbon flux forecast model was developed in this study, which was then further used to carry out carbon assimilation based on a regional chemical transport model (CMAQ) at higher spatial (64 × 64 km 2 ) and temporal (1 hr) resolutions. An Ensemble Kalman Smoother was applied as the assimilation algorithm and further extended to assimilate surface CO 2 observations. Concentrations and fluxes were simultaneously assimilated as state variables to help reduce the uncertainty in the initial CO 2 fields with the joint data assimilation framework (JDAS). In general, the posterior fluxes reproduced the seasonal, daily and hourly variation effectively, demonstrating the ability to fully absorb and utilize observations. Moreover, the influence of the choice of assimilation window on the carbon flux inversion was assessed via sensitivity experiments, revealing 36 hr to be the optimum length. Evaluation of the prior and posterior flux simulations also indicated that JDAS offers reasonable improvements, making it suitable for fine‐scale flux optimization and estimation. In addition, the posterior biosphere estimation in mainland China (−682 TgC yr −1 ) tends to be the optimal mathematical solution under current sparse observation coverage with daytime photosynthetic uptake, which likely leads to the overestimation of the optimized CO 2 sink. This study serves as a basis for future regional and urban assessment.
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