材料科学
多光谱图像
光电探测器
光电子学
钙钛矿(结构)
分辨率(逻辑)
高分辨率
纳米技术
遥感
计算机科学
人工智能
化学工程
地质学
工程类
作者
Yongqing Duan,Rui Yu,Hanyuan Zhang,Weili Yang,Wenshuo Xie,YongAn Huang,Zhouping Yin
标识
DOI:10.1002/adma.202313946
摘要
Abstract Micro/nanostructured perovskites with spatially graded compositions and bandgaps are promising in filter‐free, chip‐level multispectral, and hyperspectral detection. However, achieving high‐resolution patterning of perovskites with controlled graded compositions is challenging. Here, a programmable mixed electrohydrodynamic printing (M‐ePrinting) technique is presented to realize the one‐step direct‐printing of arbitrary spatially graded perovskite micro/nanopatterns for the first time. M‐ePrinting enables in situ mixing and ejection of solutions with controlled composition/bandgap by programmatically varying driving voltage applied to a multichannel nozzle. Composition can be graded over a single dot, line or complex pattern, and the printed feature size is down to 1 µm, which is the highest printing resolution of graded patterns to the knowledge. Photodetectors based on micro/nanostructured perovskites with halide ions gradually varying from Br to I are constructed, which successfully achieve multispectral detection and full‐color imaging, with a high detectivity and responsivity of 3.27 × 10 15 Jones and 69.88 A W −1 , respectively. The presented method provides a versatile and competitive approach for such miniaturized bandgap‐tunable perovskite spectrometer platforms and artificial vision systems, and also opens new avenues for the digital fabrication of composition‐programmable structures.
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